News & Views |
Featured
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Article |
Nuclear spin polarization and control in hexagonal boron nitride
Unlike electron spins, nuclear spins in van der Waals materials remain a largely untapped quantum resource. Here we report the fast coherent control of nuclear spins and strong electron-mediated nuclear–nuclear spin coupling in hexagonal boron nitride.
- Xingyu Gao
- , Sumukh Vaidya
- & Tongcang Li
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Letter |
Scalable optical manufacture of dynamic structural colour in stretchable materials
Desired for optical sensing or visual communications, structural colour-changing materials are hindered by the lack of scalable manufacturing. Here, by adapting Lippmann photography, large-area manufacturing of colour patterns in photosensitive elastomers is realized.
- Benjamin Harvey Miller
- , Helen Liu
- & Mathias Kolle
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News & Views |
Twistronics and the small-angle magic
Understanding, at the atomic level, the effect of the stacking and twisting of different layered two-dimensional materials is a major challenge for the future of twistronics. Optical excitations evidence twist-angle-dependent whirlpool-shaped distortions in such materials.
- Ado Jorio
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News & Views |
Intra-molecular switching for memory and logic
Individual fullerenes containing switchable electric dipoles have been demonstrated to function as single-molecule memory and logic at room temperature.
- Douglas Natelson
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Article |
Room-temperature logic-in-memory operations in single-metallofullerene devices
Single-molecule electronics provide the potential solution for high-density integration and low-power consumption in massive data-driven applications, but have yet to be explored. Here, the authors report low-power logic-in-memory operations, based on single electric dipole flipping in the two-terminal single-metallofullerene device at room temperature.
- Jing Li
- , Songjun Hou
- & Wenjing Hong
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Article |
Tuning colour centres at a twisted hexagonal boron nitride interface
Colour centre emission from hexagonal boron nitride (hBN) holds promise for quantum technologies but activation and tuning are challenging. Here, the authors show twist-angle emission brightness tuning and external voltage brightness modulation at the twisted interface of hBN flakes.
- Cong Su
- , Fang Zhang
- & Alex Zettl
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Article |
Graphene oxide bulk material reinforced by heterophase platelets with multiscale interface crosslinking
A nacre-inspired, centimetre-sized bulk material is prepared by assembling graphene oxide and microscale amorphous/crystalline heterophase reinforcing platelets adhered together with polymer-based crosslinkers, which shows high flexural strength and fracture toughness.
- Ke Chen
- , Xuke Tang
- & Lin Guo
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Article |
Emergence of correlations in alternating twist quadrilayer graphene
The twist angle dependence of correlations in alternating twist quadrilayer graphene is reported.
- G. William Burg
- , Eslam Khalaf
- & Emanuel Tutuc
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News & Views |
Nanotwinning-assisted recrystallization
Dynamic recrystallization helps to refine grain structures in metals and tune their properties. Confining recrystallization within prior nanoscale twinning provides a path for reaching exceptional grain refinement.
- Roland E. Logé
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Review Article |
Electrotunable friction with ionic liquid lubricants
This Review discusses the development of electronanotribology, its intersection with room-temperature ionic liquids and how such collaboration can be used to electrically control friction at the nanoscale.
- Fernando Bresme
- , Alexei A. Kornyshev
- & Michael Urbakh
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Article
| Open AccessUnconventional excitonic states with phonon sidebands in layered silicon diphosphide
Distinct electronic and optical properties emerge from quantum confinement in low-dimensional materials. Here, combining optical characterization and ab initio calculations, the authors report an unconventional excitonic state and bound phonon sideband in layered silicon diphosphide.
- Ling Zhou
- , Junwei Huang
- & Hongtao Yuan
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Editorial |
Materials at the heart of the COVID-19 pandemic
Materials scientists have played a key role in the global response to the COVID-19 pandemic from the development of vaccines and diagnostic tools to the rapid prototyping of ventilators.
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News & Views |
Reassembled nanoprecipitates resisting radiation
Outstanding resistance to destructive radiation damage in structural alloys is realized by ultra-high-density reversible nanoprecipitate inclusions, and the improvement is attributed to the reordering process of low-misfit superlattices in highly supersaturated matrices.
- Yanwen Zhang
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Article |
Spontaneous formation of metastable orientation with well-organized permanent dipole moment in organic glassy films
The performance of organic optoelectronic and energy-harvesting devices is largely dictated by molecular orientation and resultant permanent dipole moment. Here, the authors demonstrate a strategy to actively control dipole direction in organic glassy films.
- Masaki Tanaka
- , Morgan Auffray
- & Chihaya Adachi
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News & Views |
Wireless neuromodulation with porous silicon
Wireless optoelectronic devices are fabricated by controlling the porosity of p-type silicon, enabling in vivo efficient, non-genetic optoelectronic modulation of peripheral nerve activity.
- Silvestro Micera
- & Eugenio Redolfi Riva
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News & Views |
Bringing some bulk into ferroelectric devices
Sub-100-mV switching at the nanosecond timescale is achieved in ferroelectric devices by approaching bulk-like perfection in prototypical BaTiO3 thin films.
- Morgan Trassin
- & Vincent Garcia
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Article |
Porosity-based heterojunctions enable leadless optoelectronic modulation of tissues
Fabrication of semiconductor heterojunctions typically involves a complex process and often leads to bioincompatibility. Here, the authors propose a porous heterojunction in p-type silicon via simple stain etching at ambient conditions, and apply it in optically induced biomodulation.
- Aleksander Prominski
- , Jiuyun Shi
- & Menahem Y. Rotenberg
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Article |
Nanotwinning-assisted dynamic recrystallization at high strains and strain rates
Extreme mechanical deformation processes can lead to nanograins in many metals, but the underlying mechanism remains unclear. Nanotwinning-assisted dynamic recrystallization is shown to facilitate grain refinement to the nanoscale at high strains and strain rates.
- Ahmed A. Tiamiyu
- , Edward L. Pang
- & Christopher A. Schuh
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News & Views |
Handy nanoquakes
Electrically programmable Fourier-synthesized acoustic tweezers enable facile manipulation of micrometre-sized objects, colloids and living cells in a lab-on-chip device that combines high throughput with minimal invasive yet highly tunable force fields.
- Hubert J. Krenner
- & Christoph Westerhausen
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News & Views |
Busting through quantum dot barriers
Early time transient absorption microscopy in quantum dot solids reveals anomalous exciton transport with multiple different temporal regimes within hundreds of femtoseconds after photoexcitation.
- Naomi S. Ginsberg
- & William A. Tisdale
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Article |
Electrochemically induced amorphous-to-rock-salt phase transformation in niobium oxide electrode for Li-ion batteries
Intercalation-type metal oxides are promising anodes for Li-ion batteries but suffer from low energy and power density together with cycling instability. A nanostructured rock-salt Nb2O5 formed via amorphous-to-crystalline transformation during cycling with Li+ is shown to exhibit enhanced performance.
- Pete Barnes
- , Yunxing Zuo
- & Hui Xiong
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Article |
Anomalous optical excitations from arrays of whirlpooled lattice distortions in moiré superlattices
Recent studies have revealed unexpected characteristics in moiré superlattices formed by stacking two-dimensional crystals. Here, the authors report whirlpool-shaped periodic lattice distortions in moiré superlattices leading to anomalous optical responses.
- Jungcheol Kim
- , Eunjung Ko
- & Hyeonsik Cheong
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Letter |
Domino-like stacking order switching in twisted monolayer–multilayer graphene
The interface stacking order of twisted graphene can be actively flipped between locally stable states using a mechanical impulse, and this flipping propagates spontaneously through the network in a domino-like fashion.
- Shuai Zhang
- , Qiang Xu
- & Qunyang Li
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Article |
Renal clearable polyfluorophore nanosensors for early diagnosis of cancer and allograft rejection
Early cancer detection typically involves invasive biopsies. Here the authors designed nanosensors that are depolymerized by disease-associated enzymes in vivo to produce fluorescent urinary signals for non-invasive early diagnosis.
- Jiaguo Huang
- , Xiaona Chen
- & Kanyi Pu
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Article |
Multiscale hierarchical structures from a nanocluster mesophase
Nanometre-sized clusters can self-organize into centimetre-scale hierarchical structures, mimicking the complex constructions seen in nature and providing a platform to design synthetically directed advanced materials with sophisticated functions.
- Haixiang Han
- , Shantanu Kallakuri
- & Richard D. Robinson
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News & Views |
2D materials shrink superconducting qubits
The exceptional quality of hexagonal boron nitride crystals that can be cleaved into few layers provides ultrathin dielectrics, thereby opening a route to ultrasmall capacitors with large capacitances. With such capacitors, the superconducting transmon qubit is scaled down by orders of magnitude.
- Christian Schönenberger
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Article |
Disentangling water, ion and polymer dynamics in an anion exchange membrane
Semipermeable polymeric anion exchange membranes are essential for separation, filtration and energy conversion technologies such as fuel cells. Quasi-elastic neutron scattering is now used to disentangle water, polymer relaxation and OH− diffusional dynamics in a commercially available membrane.
- Fabrizia Foglia
- , Quentin Berrod
- & Paul F. McMillan
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Article |
Ultrafast exciton transport at early times in quantum dot solids
Understanding exciton dynamics in quantum dots is important for realizing their potential in optoelectronics. Here, the authors use femtosecond transient absorption microscopy to reveal ultrafast exciton transport, enhanced at larger interdot distance and taking place within hundreds of femtoseconds after generation.
- Zhilong Zhang
- , Jooyoung Sung
- & Akshay Rao
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Letter |
Hexagonal boron nitride as a low-loss dielectric for superconducting quantum circuits and qubits
Parallel-plate capacitors of the two-dimensional materials hBN and NbSe2 are integrated with aluminium Josephson junctions to realize transmon qubits with coherence times reaching 25 μs.
- Joel I-J. Wang
- , Megan A. Yamoah
- & William D. Oliver
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Article |
Geometrically stabilized skyrmionic vortex in FeGe tetrahedral nanoparticles
The real-space magnetic configurations of a zero-dimensional skyrmionic vortex structure is uncovered using electron holography and micromagnetic simulations.
- Kodai Niitsu
- , Yizhou Liu
- & Yoshinori Tokura
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Article |
Tandem catalysis with double-shelled hollow spheres
Metal oxide–zeolite bifunctional catalysts allow coupling of reactions and so enhance catalytic processes, but structure and reactivity control is difficult. Here, a general synthesis is presented for metal oxide–zeolite double-shelled hollow spheres, which outperform other catalysts for petroleum production.
- Jiadong Xiao
- , Kang Cheng
- & Bert M. Weckhuysen
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Article |
Suspension electrolyte with modified Li+ solvation environment for lithium metal batteries
Stable solid–electrolyte interphases on Li anodes are crucial for reliable Li metal batteries. A suspension electrolyte design that modifies the Li+ solvation environment in liquid electrolytes and creates inorganic-rich interphases on Li is now reported.
- Mun Sek Kim
- , Zewen Zhang
- & Yi Cui
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Article |
The emergence of valency in colloidal crystals through electron equivalents
Symmetry breaking in colloidal crystals is achieved with DNA-grafted programmable atom equivalents and complementary electron equivalents, whose interactions are tuned to create anisotropic crystalline precursors with well-defined coordination geometries that assemble into distinct low-symmetry crystals.
- Shunzhi Wang
- , Sangmin Lee
- & Chad A. Mirkin
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Article |
Inter-facet junction effects on particulate photoelectrodes
In anisotropically shaped photocatalyst particles different constituent facets may form inter-facet junctions at their adjoining edges. Using multimodal functional imaging, inter-facet junction effects on anisotropically shaped bismuth vanadate particles are revealed.
- Xianwen Mao
- & Peng Chen
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News & Views |
Sliding on the edge
Heterogeneous microscale contacts between molybdenum disulfide and graphene or hexagonal boron nitride layers demonstrate ultralow friction independent of their relative orientation with residual drag that originates from edge effects.
- Oded Hod
- & Michael Urbakh
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Article |
Memristive control of mutual spin Hall nano-oscillator synchronization for neuromorphic computing
This allows versatile non-volatile tuning of the mutual synchronization of chains of up to four oscillators and provides a path toward individual oscillator control in large oscillatory arrays.
- Mohammad Zahedinejad
- , Himanshu Fulara
- & Johan Åkerman
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Article |
Atomic-scale observation of non-classical nucleation-mediated phase transformation in a titanium alloy
A full kinetic pathway of a non-classical nucleation-induced phase transformation through metastable states is elucidated at sub-ångström resolution in a technologically important titanium alloy.
- Xiaoqian Fu
- , Xu-Dong Wang
- & En Ma
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Article |
Fabrication and nanophotonic waveguide integration of silicon carbide colour centres with preserved spin-optical coherence
Colour centres are a promising quantum information platform, but coherence degradation after integration in nanostructures has hindered scalability. Here, the authors show that waveguide-integrated VSi centres in SiC maintain spin-optical coherences, enabling nuclear high-fidelity spin qubit operations.
- Charles Babin
- , Rainer Stöhr
- & Jörg Wrachtrup
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Article |
Interface polarization in heterovalent core–shell nanocrystals
Controlled synthesis of heterostructured III-V–II-VI nanocrystals shows that dipole moments formed at the core–shell interface can tune the optoelectronic properties of these nanomaterials and their performance in light-emitting devices.
- Byeong Guk Jeong
- , Jun Hyuk Chang
- & Wan Ki Bae
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News & Views |
Nano goes the distance
Centimetre-scale crack-free metal nanolattices are realized, enabling outstanding high tensile strength in low-density materials.
- Andreas Stein
- & Nathan A. Mara
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Article |
Ultra-low-density digitally architected carbon with a strutted tube-in-tube structure
A nanoscale tube-in-tube sandwich structure is generated by a two-step templating-pyrolysis process, which strengthens the log-pile carbon architecture and slows down the decrease of stiffness with decreasing density.
- Jianchao Ye
- , Ling Liu
- & Juergen Biener
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Article |
Deterministic inverse design of Tamm plasmon thermal emitters with multi-resonant control
Tamm plasmon thermal emitters can provide low-cost, efficient mid to long infrared emission, but have been limited by a challenging design. Here the authors apply an inverse design protocol to demonstrate tailorable multi-band emission on CdO films.
- Mingze He
- , J. Ryan Nolen
- & Joshua D. Caldwell
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Article |
3D-printed silica with nanoscale resolution
A 3D-printing technique has been developed to create high-quality pure silica nanostructures with sub-200 nm resolution and the flexible capability of rare-earth element doping. It shows excellent application potential in three-dimensional micro- and nanophotonics.
- Xiewen Wen
- , Boyu Zhang
- & Jun Lou
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News & Views |
The secret order of disorder
A seemingly disordered network of nanowires governed by thermodynamics is used as the physical ‘reservoir’ in a memristive implementation of reservoir computing to process spatiotemporal information.
- Qiangfei Xia
- , J. Joshua Yang
- & Rivu Midya
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Article |
In materia reservoir computing with a fully memristive architecture based on self-organizing nanowire networks
A network of self-organized nanowires combined with a memristive read-out layer is used to demonstrate a hardware implementation of reservoir computing for recognition of spatio-temporal patterns and time-series prediction.
- Gianluca Milano
- , Giacomo Pedretti
- & Carlo Ricciardi
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Article |
Giant magnetoelastic effect in soft systems for bioelectronics
Micromagnets dispersed in a polymer matrix are used to realize a soft magnetoelastic generator with high magnetomechanical coupling factor, used for wearable and implantable power generation and sensing applications.
- Yihao Zhou
- , Xun Zhao
- & Jun Chen
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News & Views |
A ‘Swiss army knife’ probe for metastatic cancers
A nanosensor probe that combines a tumour-targeting peptide, a diagnostic reporter and an imaging contrast agent enables early diagnosis, precision imaging, disease stratification and downstream therapeutic response monitoring of metastatic cancer.
- Matthew Bogyo
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Article |
Site-specific chemical doping reveals electron atmospheres at the surfaces of organic semiconductor crystals
Organic semiconductor crystals can be selectively doped at the crystallographic step edges, deactivating shallow traps and recovering band-like transport. The space charge induced by chemical doping is observed by scanning Kelvin probe microscopy.
- Tao He
- , Matthias Stolte
- & C. Daniel Frisbie
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Article |
Ion exchange in atomically thin clays and micas
Layered clays are of interest for membranes and many other applications but their ion-exchange dynamics remain unexplored in atomically thin materials. Here, using electron microscopy, it is found that the ion diffusion for few-layer two-dimensional clays approaches that of free water and that superlattice cation islands can form in twisted and restacked materials.
- Yi-Chao Zou
- , Lucas Mogg
- & Sarah J. Haigh