Optics and photonics articles within Nature Materials

Featured

  • Article |

    Combining resonant inelastic X-ray scattering and photoluminescence spectroscopy, an elementary excitation in hexagonal-boron-nitride-based single-photon emitters has been demonstrated, giving rise to multiple regular harmonics that can explain the wide frequency range of these emitters.

    • Jonathan Pelliciari
    • , Enrique Mejia
    •  & Gabriele Grosso
  • Article |

    Lack of local phase patterning in liquid crystal elastomers has hindered their broad implementation. The authors report a laser-induced dynamic crosslinking approach with allyl sulfide groups to achieve reconfigurable high-resolution patterning of multiple liquid crystalline phases in a single film.

    • Seok Hwan Choi
    • , Ju Hee Kim
    •  & Seung Hwan Ko
  • News & Views |

    Cancer cells adjust the composition of their glycocalyx to increase its thickness and create a physical barrier that shields them from immune recognition and engagement.

    • Edward N. Schmidt
    •  & Matthew S. Macauley
  • Article
    | Open Access

    The authors propose a non-Hermitian topological insulator with a real-valued energy spectrum based on a periodically driven Floquet model implemented in a photonic platform where generalized parity–time symmetry is protected against spontaneous symmetry breaking under a spatiotemporal gain and loss distribution.

    • Alexander Fritzsche
    • , Tobias Biesenthal
    •  & Alexander Szameit
  • Article |

    Propagation losses have limited the practical use of polaritons in photonic applications. Here the authors demonstrate a substantial enhancement in the propagation distance of phonon polaritons, employing synthetic optical excitation of complex frequency with virtual gain synthesized by combining multiple real frequency measurements.

    • Fuxin Guan
    • , Xiangdong Guo
    •  & Shuang Zhang
  • Article |

    Employing light-transformable polymers, multiple physical unclonable functions are demonstrated within a single device with all-optical reversible reconfigurability. Such devices may enable quantum secure authentication and nonlinear cryptographic key generation applications.

    • Sara Nocentini
    • , Ulrich Rührmair
    •  & Francesco Riboli
  • Research Briefing |

    Hybrid organic–inorganic perovskite materials have promise as the photovoltaic technology of the future. A method for spectroscopic optical control reveals how the structural dynamics and vibrations of a perovskite’s organic cations affect the electronic performance of working photovoltaic devices.

  • News & Views |

    Hybridized electron or hole states across semiconducting van der Waals monolayers in heterotrilayer systems enable the emergence of quadrupolar excitons. Quadrupolar excitons, unlike their dipolar counterparts, have a tunable static dipole moment that responds nonlinearly under an applied electric field.

    • Elyse Barré
    • , Medha Dandu
    •  & Archana Raja
  • Article
    | Open Access

    Optically stimulated vibrational control for materials has the potential to improve the performance of optoelectronic devices. The vibrational control of FAPbBr3 perovskite solar cells has been demonstrated, where the fast dynamics of coupling between cations and inorganic sublattice may suppress non-radiative recombinations in perovskites, leading to reduced voltage losses.

    • Nathaniel. P. Gallop
    • , Dmitry R. Maslennikov
    •  & Artem A. Bakulin
  • Article |

    Employing a miniaturized spectrometer that combines a metasurface-based spectrometer array and a metalens, angle-resolved spectral imaging is achieved with a wavelength accuracy of 0.17 nm, spectral resolution of 0.40 nm and angular resolution of 4.88 × 10−3 rad for a spectrometer with a 4 × 4 μm2 footprint.

    • Guiyi Cai
    • , Yanhao Li
    •  & Qinghai Song
  • News & Views |

    Quantum dots couple to form artificial molecules that allow for variable colour emission in response to an electric field.

    • James Cassidy
    • , Justin Ondry
    •  & Dmitri V. Talapin
  • Research Briefing |

    Inspired by valley pseudospins in two-dimensional materials, high-quality-factor (high-Q) spin–valley states were created through the photonic Rashba-type spin splitting of a bound state in the continuum. This approach enabled the construction of a coherent and controllable spin-optical laser using monolayer-integrated spin–valley microcavities without requiring magnetic fields or cryogenic temperatures.

  • Research Briefing |

    By optimizing the molecular organization of blue-emitting organic semiconductors, the vulnerability of the materials to extrinsic impurities that cause charge trapping, such as oxygen and water, is strongly reduced. Steric shielding of the electron-transporting core is shown to increase the electron transport by several orders of magnitude.

  • News & Views |

    Quantum dots are engineered to use dopant states to achieve substantially enhanced impact ionization, which is potentially useful for light-harvesting applications.

    • Miri Kazes
    •  & Dan Oron
  • Article
    | Open Access

    Carrier multiplication generates multiple excitons for each absorbed photon but is normally limited by fast phonon-assisted relaxation. Here the authors achieve a threefold enhancement in multiexciton yields in Mn-doped PbSe/CdSe quantum dots, due to very fast spin-exchange interactions between Mn ions and the quantum dots that outpace energy losses arising from phonon emission.

    • Ho Jin
    • , Clément Livache
    •  & Victor I. Klimov
  • Article |

    The authors introduce a spin-optical laser based on a monolayer transition metal dichalcogenide coupled to a heterostructure microcavity supporting high-Q spin-valley resonances originating from photonic Rashba-type spin splitting of a bound state in the continuum.

    • Kexiu Rong
    • , Xiaoyang Duan
    •  & Erez Hasman
  • Research Briefing |

    High-quality aluminium nitride (AlN) heteroepitaxial films are obtained by the controlled discretization and coalescence of columns using nanopatterned AlN/sapphire templates with regular hexagonal holes. The density of dislocation etch pits in the AlN heteroepitaxial films is reduced to approximately 104 cm–2, approaching the value of that in AlN bulk single crystals.

  • Research Briefing |

    A scalar scheme has been proposed to design photonic crystals that possess bulk dispersions resembling scalar waves and surface modes that support skyrmion-like textures. This approach addresses the challenges of realizing three-dimensional topological photonic crystals, which usually have complicated dispersions and leaky surface modes inside the light cone.

  • Article |

    The direction of polariton canalization—its diffractionless propagation—in twisted bilayers at the magic angle is hindered by the lack of multiple magic angles. By controlling the twist angles between three α-MoO3 layers, reconfigurable and spectrally robust polariton canalization along any in-plane direction is demonstrated.

    • J. Duan
    • , G. Álvarez-Pérez
    •  & P. Alonso-González
  • News & Views |

    Current-inducing switching of magnetization is crucial for future magnetic data processing technologies, but switching it with speed and energy efficiency remains challenging. Using femtosecond optical pulses, instead of conventional charge currents, is found to make spintronics not only ultrafast but also counterintuitive.

    • Dmytro Afanasiev
    •  & Alexey V. Kimel
  • News & Views |

    Above-bandgap, nanosecond laser pulses enable the localized in situ writing of spin defects in prefabricated nanophotonic cavities. The approach preserves defect and cavity mode properties, key requirements towards cavity–emitter coupling in quantum networks.

    • Sridhar Majety
    •  & Marina Radulaski
  • Letter
    | Open Access

    The authors report subatomic precision in measuring the displacement of a nanowire. Such precision is achieved by employing deep-learning enabled analysis of single-shot scattering of topologically structured superoscillatory illumination.

    • Tongjun Liu
    • , Cheng-Hung Chi
    •  & Nikolay I. Zheludev
  • Letter |

    Using direct laser writing with a nanosecond pulsed laser operating at above-bandgap photon energies, we demonstrate the selective formation of spin defects in photonic crystal cavities in 4H-silicon carbide and their in situ characterization.

    • Aaron M. Day
    • , Jonathan R. Dietz
    •  & Evelyn L. Hu
  • Letter |

    We report compact spin-valley-locked perovskite emitting metasurfaces where spin-dependent geometric phases are imparted into bound states in the continuum via Brillouin zone folding, simultaneously enabling chiral purity, directionality and large emission angles.

    • Yang Chen
    • , Jiangang Feng
    •  & Cheng-Wei Qiu
  • Article |

    The authors demonstrate electrical on/off switching of interlayer interactions in tungsten diselenide/molybdenum disulfide heterobilayers, the phase diagram of which contains layer-dependent correlated regions that reveal the role of strong correlations in interlayer exciton dynamics.

    • Qinghai Tan
    • , Abdullah Rasmita
    •  & Weibo Gao
  • Letter |

    Employing an oxidation-activated charge transfer strategy to oxidize transition-metal dichalcogenides into transition-metal oxides, the authors imprint plasmonic cavities with laterally abrupt doping profiles and nanoscale precision demonstrating plasmonic whispering-gallery resonators.

    • Brian S. Y. Kim
    • , Aaron J. Sternbach
    •  & D. N. Basov
  • News & Views |

    Time-dependent pump–probe studies of polaritonic transport — for polaritons formed by strong coupling between organic molecules and Bloch surface waves at the interface of a distributed Bragg reflector — reveal a transition between diffusive and ballistic behaviour.

    • Jonathan Keeling
    •  & Graham Turnbull
  • Article |

    The authors report spin current generation in a metallic layer adjacent to a non-magnetic chiral hybrid organic–inorganic perovskite when subjected to a thermal gradient, and attribute this to chiral phonons possessing angular momentum.

    • Kyunghoon Kim
    • , Eric Vetter
    •  & Jun Liu
  • Article |

    On-demand electron wavefront shaping is desirable for applications from nanolithography to imaging. Here, the authors present tunable photon-induced spatial modulation of electrons through their interaction with externally controlled surface plasmon polaritons.

    • Shai Tsesses
    • , Raphael Dahan
    •  & Ido Kaminer
  • Article |

    Liquid crystal (LC) applications typically rely on defining the non-topological spatial patterns of the optical axis. Here, the authors demonstrate the topological steering of light by LC nematic vortices, futher establishing an analogy between topological light steering by LC vortices and cosmic strings.

    • Cuiling Meng
    • , Jin-Sheng Wu
    •  & Ivan I. Smalyukh
  • Article
    | Open Access

    Triplet-fusion-based photon upconversion is promising for photovoltaic or bioimaging applications, but its efficiency is limited by triplet fusion spin dependence. Here, the authors tailor spin dynamics by engineering the crystal structure with metal–organic frameworks to enable effective spin mixing between singlet and quintet triplet–triplet pair states.

    • Dong-Gwang Ha
    • , Ruomeng Wan
    •  & Mircea Dincă
  • Article |

    The authors use circularly polarized light pulses to trigger all-optical magnetization switching in an atomically thin ferromagnetic semiconductor. The switching process is related to spin angular momentum transfer from photoexcited carriers to local magnetic moments.

    • Peiyao Zhang
    • , Ting-Fung Chung
    •  & Xiang Zhang
  • News & Views |

    Ensemble-level experimental evidence of exciton fine-structure splitting in perovskite quantum dots has been demonstrated, correlated to the intrinsic symmetry of these nanocrystals.

    • Gabriele Rainò
    •  & Maksym V. Kovalenko
  • News & Views |

    By exploiting subfemtosecond control of light pulses, researchers demonstrate an ultrafast logic gate based on the waveform-dependent photocurrent generated by real and virtual carriers in graphene.

    • Klaas-Jan Tielrooij
  • Comment |

    The success of silicon photonics is a product of two decades of innovations. This photonic platform is enabling novel research fields and novel applications ranging from remote sensing to ultrahigh-bandwidth communications. The future of silicon photonics depends on our ability to ensure scalability in bandwidth, size and power.

    • Michal Lipson