Featured
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Article |
Scalable integration of hybrid high-κ dielectric materials on two-dimensional semiconductors
A van der Waals buffer layer of Sb2O3 enables the integration of high-κ dielectric layer with sub-1 nm equivalent oxide thickness on two-dimensional semiconductors, resulting in high performance of two-dimensional field-effect transistors.
- Yongshan Xu
- , Teng Liu
- & Tianyou Zhai
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News & Views |
Dancing with an electric field
An electric field is found to be capable of controlling dislocation movement in semiconducting zinc sulfide, as observed in real time by in situ transmission electron microscopy.
- Xufei Fang
- & Jürgen Rödel
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Research Briefing |
Mapping the transmission of single-molecule junctions using photoelectron tunnelling spectroscopy
The transmission spectrum of single-molecule junctions provides fingerprint information on the charge-transport properties. A technique called single-molecule photoelectron tunnelling spectroscopy has been developed that enables mapping of the transmission spectrum beyond the highest occupied molecular orbital (HOMO)–lowest unoccupied molecular orbital (LUMO) gap at room temperature and can be used to explore the energy-dependent charge transport through single-molecule junctions.
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News & Views |
A new spin on impact ionization
Quantum dots are engineered to use dopant states to achieve substantially enhanced impact ionization, which is potentially useful for light-harvesting applications.
- Miri Kazes
- & Dan Oron
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Article |
Direct growth of single-chiral-angle tungsten disulfide nanotubes using gold nanoparticle catalysts
The direct and facile growth of WS2 and WSe2 nanotubes with controllable chirality is realized using catalytic chemical vapour deposition with Au nanoparticles.
- Qinwei An
- , Wenqi Xiong
- & Shengjun Yuan
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Article
| Open AccessSpin-exchange carrier multiplication in manganese-doped colloidal quantum dots
Carrier multiplication generates multiple excitons for each absorbed photon but is normally limited by fast phonon-assisted relaxation. Here the authors achieve a threefold enhancement in multiexciton yields in Mn-doped PbSe/CdSe quantum dots, due to very fast spin-exchange interactions between Mn ions and the quantum dots that outpace energy losses arising from phonon emission.
- Ho Jin
- , Clément Livache
- & Victor I. Klimov
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Article
| Open AccessExciton-assisted electron tunnelling in van der Waals heterostructures
The authors demonstrate exciton-assisted resonant electron tunnelling in van der Waals heterostructure tunnel junctions. Their study elucidates tunnelling mechanisms involving either indirect or direct excitons in the absence of charge injection and reveals excitonic light emission driven by inelastic electron tunnelling.
- Lujun Wang
- , Sotirios Papadopoulos
- & Lukas Novotny
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News & Views |
A twist for nanolight
Controlling the twist angles between three α-phase molybdenum trioxide single layers enables the programmable and reconfigurable canalization of phonon polaritons along multiple in-plane directions.
- Siyuan Dai
- & Qiong Ma
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Article
| Open AccessIntrinsic strong light-matter coupling with self-hybridized bound states in the continuum in van der Waals metasurfaces
The authors demonstrate strong coupling in bound state in the continuum metasurfaces on nanostructured bulk WS2 and exhibiting sharp resonances with tailored linewidths and controllable light-matter coupling strength.
- Thomas Weber
- , Lucca Kühner
- & Andreas Tittl
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Article |
Amorphous nickel hydroxide shell tailors local chemical environment on platinum surface for alkaline hydrogen evolution reaction
Elaborated catalysts design can substantially enhance performance under unfavourable reaction conditions. Amorphous nickel hydroxide proton sieve used to modify local chemical environment on a platinum surface results in unprecedented performance for alkaline hydrogen evolution reaction.
- Chengzhang Wan
- , Zisheng Zhang
- & Xiangfeng Duan
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Article |
Single-molecule photoelectron tunnelling spectroscopy
The transmission spectrum reflects energy alignment between electrodes and frontier orbitals in single-molecule junctions but few experimental tools exist for characterization beyond the HOMO–LUMO gap. Here, the authors develop a single-molecule photoelectron tunnelling spectroscopy approach that makes it possible to map the transmission spectrum beyond the HOMO–LUMO gap at room temperature.
- Haojie Liu
- , Lijue Chen
- & Wenjing Hong
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Article |
Multiple and spectrally robust photonic magic angles in reconfigurable α-MoO3 trilayers
The direction of polariton canalization—its diffractionless propagation—in twisted bilayers at the magic angle is hindered by the lack of multiple magic angles. By controlling the twist angles between three α-MoO3 layers, reconfigurable and spectrally robust polariton canalization along any in-plane direction is demonstrated.
- J. Duan
- , G. Álvarez-Pérez
- & P. Alonso-González
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News & Views |
Writing above the bandgap
Above-bandgap, nanosecond laser pulses enable the localized in situ writing of spin defects in prefabricated nanophotonic cavities. The approach preserves defect and cavity mode properties, key requirements towards cavity–emitter coupling in quantum networks.
- Sridhar Majety
- & Marina Radulaski
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Article |
Strongly enhanced light–matter coupling of monolayer WS2 from a bound state in the continuum
Combining a tungsten disulfide monolayer and a topologically protected bound state in the continuum formed by a one-dimensional photonic crystal, strong light–matter interaction enhancement and large exciton–polariton nonlinearities at room temperature are demonstrated.
- Eugenio Maggiolini
- , Laura Polimeno
- & Dario Ballarini
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Letter
| Open AccessPicophotonic localization metrology beyond thermal fluctuations
The authors report subatomic precision in measuring the displacement of a nanowire. Such precision is achieved by employing deep-learning enabled analysis of single-shot scattering of topologically structured superoscillatory illumination.
- Tongjun Liu
- , Cheng-Hung Chi
- & Nikolay I. Zheludev
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News & Views |
Distinguishing atomic vibrations near point defects
Local vibrational modes at substitutional impurities in monolayer graphene are resolved with a sensitivity at the chemical bonding level, revealing the impacts of different chemical configurations and mass of impurity atoms on the defect-perturbed vibrational properties.
- Xingxu Yan
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Perspective |
Lessons from hafnium dioxide-based ferroelectrics
The discovery of ferroelectric switching in ultrathin layers of hafnium dioxide has aroused significant interest for low-power non-volatile memory technologies. This Perspective discusses how lessons learned from hafnium dioxide-based ferroelectrics can be applied to other applications, and other binary oxides.
- Beatriz Noheda
- , Pavan Nukala
- & Mónica Acuautla
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Letter |
Laser writing of spin defects in nanophotonic cavities
Using direct laser writing with a nanosecond pulsed laser operating at above-bandgap photon energies, we demonstrate the selective formation of spin defects in photonic crystal cavities in 4H-silicon carbide and their in situ characterization.
- Aaron M. Day
- , Jonathan R. Dietz
- & Evelyn L. Hu
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News & Views |
Correlated states shine brighter
An optical spectroscopy approach unravels different layer-dependent correlated electron phases in a two-dimensional semiconductor heterobilayer.
- Mauro Brotons-Gisbert
- & Brian D. Gerardot
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Letter |
Ambipolar charge-transfer graphene plasmonic cavities
Employing an oxidation-activated charge transfer strategy to oxidize transition-metal dichalcogenides into transition-metal oxides, the authors imprint plasmonic cavities with laterally abrupt doping profiles and nanoscale precision demonstrating plasmonic whispering-gallery resonators.
- Brian S. Y. Kim
- , Aaron J. Sternbach
- & D. N. Basov
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Article |
Scalable manufacturing of high-index atomic layer–polymer hybrid metasurfaces for metaphotonics in the visible
The authors propose a method for the scalable manufacturing of metalenses using deep-ultraviolet argon fluoride immersion lithography and wafer-scale nanoimprint lithography, opening a route towards their low-cost, high-throughput mass production.
- Joohoon Kim
- , Junhwa Seong
- & Junsuk Rho
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Article |
Curvature-sensing peptide inhibits tumour-derived exosomes for enhanced cancer immunotherapy
A curvature-sensing antiviral peptide is repurposed to disrupt tumour-derived exosomes and used in combination with immune checkpoint blockade cancer therapy.
- Sol Shin
- , Hyewon Ko
- & Jae Hyung Park
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Review Article |
Hydrogels for RNA delivery
RNA-based therapeutics hold promise for the treatment of several diseases. This Review provides an overview of hydrogels for RNA delivery, discussing how the chemical nature and physical properties of hydrogels can be explored for tailored RNA loading and release, and highlighting the use of these materials in biomedical applications.
- Ruibo Zhong
- , Sepehr Talebian
- & Jinjun Shi
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Article |
Tip-induced excitonic luminescence nanoscopy of an atomically resolved van der Waals heterostructure
Tip-induced excitonic luminescence nanoscopy of an atomically resolved van der Waals heterostructure.
- Luis E. Parra López
- , Anna Rosławska
- & Guillaume Schull
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Article |
Single-atom vibrational spectroscopy with chemical-bonding sensitivity
Vibrational spectroscopy now allows for the exploration of lattice vibrational properties at the chemical-bond level, revealing the impact of chemical-bonding configurations and atomic mass on local phonon modes in graphene with a new level of sensitivity.
- Mingquan Xu
- , De-Liang Bao
- & Wu Zhou
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Letter |
Single-crystalline van der Waals layered dielectric with high dielectric constant
Large-size single-crystal van der Waals layered Bi2SeO5 has been synthesized with a high dielectric constant and high breakdown field strength for two-dimensional electronics applications.
- Congcong Zhang
- , Teng Tu
- & Hailin Peng
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News & Views |
Exploiting endothelial transcytosis to reach into the brain
Targeting P-selectin enables safer and more effective nanomedicine delivery through caveolin-1-mediated endothelial transcytosis in preclinical medulloblastoma tumour models.
- Lin Wang
- & Stefan Wilhelm
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News & Views |
Immunostimulatory nanoparticles go viral
A polymeric nanoparticle adjuvant containing a Toll-like receptor 7 agonist elicits broad protection against viral challenges.
- Jorge Huete-Carrasco
- & Ed C. Lavelle
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News & Views |
Ultrafast plasmonics shapes electron beams
By exploiting optical phase-modulation at complex surface plasmon polariton patterns, as well as energy-filtered imaging, femtosecond electron pulses are dynamically shaped in phase and amplitude.
- Armin Feist
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Review Article |
Controlling persistent luminescence in nanocrystalline phosphors
Persistent luminescent phosphors are promising for applications from bioimaging to multilevel encryption. Here, the authors review the design and preparation of persistent luminescence nanomaterials, developments in biological applications and outstanding challenges.
- Liangliang Liang
- , Jiaye Chen
- & Xiaogang Liu
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Article
| Open AccessP-selectin-targeted nanocarriers induce active crossing of the blood–brain barrier via caveolin-1-dependent transcytosis
Targeting of tumour vasculature endothelial P-selectin promotes caveolin-1-mediated transcytosis for enhanced blood–brain barrier crossing of therapeutic nanoparticles against medulloblastoma.
- Daniel E. Tylawsky
- , Hiroto Kiguchi
- & Daniel A. Heller
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Article
| Open AccessA TLR7-nanoparticle adjuvant promotes a broad immune response against heterologous strains of influenza and SARS-CoV-2
A nanoparticle-based adjuvant incorporating a Toll-like receptor 7 agonist elicits cross-reactive antibodies for both dominant and subdominant epitopes and enhances immune responses against multiple variants of influenza and SARS-CoV-2.
- Qian Yin
- , Wei Luo
- & Mark M. Davis
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Perspective |
Nanocrystal phononics
Colloidal nanocrystals can form into periodic superlattices exhibiting collective vibrations from the correlated motion of the nanocrystals. This Perspective discusses such collective vibrations and their as-of-yet untapped potential applications for phononic crystals, acoustic metamaterials and optomechanical systems.
- Maximilian Jansen
- , William A. Tisdale
- & Vanessa Wood
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News & Views |
Asymmetry in the magnetic neighbourhood
Transforming atomically thin materials by their magnetic neighbours reveals a surprising asymmetry that allows a versatile control of the valley degrees of freedom and band topology in van der Waals heterostructures.
- Tong Zhou
- & Igor Žutić
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Letter |
Asymmetric magnetic proximity interactions in MoSe2/CrBr3 van der Waals heterostructures
The authors demonstrate that magnetic proximity interactions in a hexagonal boron nitride-encapsulated MoSe2/CrBr3 van der Waals heterostructure have a striking difference in the two (K, K′) valleys of a monolayer MoSe2.
- Junho Choi
- , Christopher Lane
- & Scott A. Crooker
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Article |
Granular aluminium nanojunction fluxonium qubit
The authors fabricate a fluxonium circuit using a granular aluminium nanoconstriction to replace the conventional superconductor–insulator–superconductor tunnel junction. Their characterization suggests that this approach will be a useful element in the superconducting qubit toolkit.
- D. Rieger
- , S. Günzler
- & I. M. Pop
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News & Views |
The Wulff construction goes low-symmetry
An apparent quirk of mathematics draws on a symmetry and resolves the issue of how to determine the equilibrium shape of crystals of two-dimensional materials with asymmetric terminations.
- Paul Erhart
- & J. Magnus Rahm
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News & Views |
Molecular electronics go synaptic
Coupling charge transfer with molecular protonation processes yields electronic systems that display negative differential conductance, an effect that can be harnessed to implement a wide range of device configurations from logic gates to synaptic behaviour.
- Joshua Hihath
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Article |
Dynamic molecular switches with hysteretic negative differential conductance emulating synaptic behaviour
To realize electronic operations beyond the von Neumann bottleneck, a new type of switch that can mimic self-learning is needed. Here, the authors demonstrate all-in-one-place logic and memory operations based on dynamic molecular switch that can emulate brain-like synaptic and Pavlovian response, bringing the field a step closer to molecular-scale hardware.
- Yulong Wang
- , Qian Zhang
- & Christian A. Nijhuis
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Letter |
Planar thermal Hall effect of topological bosons in the Kitaev magnet α-RuCl3
The authors report a strongly temperature-dependent thermal conductivity at low temperature, consistent with topological bosonic modes in a Chern-insulator-like model.
- Peter Czajka
- , Tong Gao
- & N. P. Ong
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Article |
Hierarchically engineered nanostructures from compositionally anisotropic molecular building blocks
Independently tailored nano- and mesoscale features are obtained in hierarchically assembled mixed graft block copolymers with precisely defined side-chain sequences.
- Ruiqi Liang
- , Yazhen Xue
- & Mingjiang Zhong
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News & Views |
Twisted growth by design
Twisted bilayer graphene is epitaxially grown between two adjacent Cu(111) surfaces, with the twist angle controlled by the rotation of the Cu foils as designed.
- Seong-Jun Yang
- & Cheol-Joo Kim
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Letter |
Manipulating the insulator–metal transition through tip-induced hydrogenation
The authors realize local and reversible hydrogenation of VO2 using a Pt-coated scanning probe microscope tip and forming gas.
- Linglong Li
- , Meng Wang
- & Pu Yu
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News & Views |
Sieving in order
Designing highly ordered and ultrathin nanoporous membranes achieves superior water flux, while maintaining high selectivity for NaCl rejection.
- Chrystelle Salameh
- & Damien Voiry
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Letter |
Giant magnon spin conductivity in ultrathin yttrium iron garnet films
The authors report the observation of an enhanced magnon conductivity close to the two-dimensional transport regime in ultrathin yttrium iron garnet.
- X.-Y. Wei
- , O. Alves Santos
- & B. J. van Wees
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Article |
Nanoparticle-modified microrobots for in vivo antibiotic delivery to treat acute bacterial pneumonia
Biohybrid microrobots consisting of nanoparticle-modified microalgae are constructed for active drug delivery in the lungs. In an acute bacterial pneumonia model, the microrobots effectively reduce bacterial burden and lessen animal mortality.
- Fangyu Zhang
- , Jia Zhuang
- & Joseph Wang
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Article |
Designed growth of large bilayer graphene with arbitrary twist angles
Angle tunability in twisted bilayer graphene is crucial in promoting its applications of twistronics. Here an angle replication strategy is developed to obtain centimetre-scale bilayer graphene with arbitrary twist angles.
- Can Liu
- , Zehui Li
- & Kaihui Liu
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News & Views |
Locking exciton fine-structure splitting
Ensemble-level experimental evidence of exciton fine-structure splitting in perovskite quantum dots has been demonstrated, correlated to the intrinsic symmetry of these nanocrystals.
- Gabriele Rainò
- & Maksym V. Kovalenko
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Article |
Lattice distortion inducing exciton splitting and coherent quantum beating in CsPbI3 perovskite quantum dots
Halide perovskites feature highly dynamic lattices, but their impact on exciton fine structure remains unexplored. Here, the authors show that these lattices lead to a bright-exciton fine structure gap, enabling observation of quantum beats in a non-uniform ensemble.
- Yaoyao Han
- , Wenfei Liang
- & Kaifeng Wu