Abstract
A binary switch is the basic building block for information processing. The potential energy profile of a bistable binary switch is a ‘symmetric’ double well. The traditional method of switching it from one state (one well) to the other is to tilt the profile towards the desired state. Here, we present a case, where no such tilting is necessary to switch successfully, even in the presence of thermal noise. This happens because of the built-in dynamics inside the switch itself. It differs from the general perception on binary switching that in a ‘symmetric’ potential landscape, the switching probability is 50% in the presence of thermal noise. Our results, considering the complete three-dimensional potential landscape, demonstrate intriguing phenomena on binary switching mechanism. With experimentally feasible parameters, we theoretically demonstrate such intriguing possibility in electric field induced magnetization switching of a shape-anisotropic single-domain magnetostrictive nanomagnet with two stable states at room-temperature.
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Introduction
Understanding the operation of a binary switch, i.e., how switching takes place from one stable state to another, enables us to design a better switch to meet our ever-increasing demand to store, process, and communicate information. From around mid-nineties, the methodology of basic binary switching for information processing as conceived by famous scientist Landauer and others is based on the fact that an externally introduced tilt or asymmetry in the potential landscape of a bistable element in the desired direction of switching is necessary1,2,3,4. This can be achieved by utilizing an external magnetic field in an elliptical single-domain nanomagnet with two stable magnetization states along the ellipse's major axis acting as a binary switch4. The magnetic field, directed along the desired direction of switching, results in a ‘tilt’ in the magnet's double-well potential profile and this tilt generates a motion along the direction of switching. As long as the tilt is sufficient to beat the thermal agitations, switching with a tolerable error probability is achieved. Such tilt or asymmetry in potential landscape is usually deemed to be necessary for switching to take place. Fig. 1a depicts such traditional methodology of binary switching.
We point out here that the magnetization switching mechanism using spin-transfer-torque5,6, in which a spin-polarized current is passed through a nanomagnet, is analogous to the traditional methodology. Even if the spin-transfer-torque has a component that cannot be absorbed as an effective potential5, the direction of the externally applied spin-polarized current creates an equivalent tilt or asymmetry causing the switching in the desired direction. However, magnetization reversal is possible by spin-torque induced precessional motion7,8 as well as by the electric field induced magnetic anisotropy9,10. There is also mechanism of bidirectional electron pump based on Coulomb blockade in single electron tunneling devices11,12.
In this article, we show that no such tilting of potential landscape of the bistable switch by external means is necessary to switch successfully, even in the presence of thermal noise. Fig. 1b illustrates the basic concept underlying the proposed methodology of binary switching. We consider the complete three-dimensional potential landscape and demonstrate that the internal dynamics can provide an equivalent asymmetry without any requirement of making the potential landscape asymmetric. Note that for both the cases (traditional and proposed methodologies), it is necessary to lower the energy barrier and make the monostable well deep enough to withstand thermal fluctuations. For a magnetostrictive nanomagnet on which our study is based, stress is the external agent inverting the potential landscape. The stress can be generated on a magnetostrictive nanomagnet by applying a voltage on a piezoelectric layer elastically coupled to it, i.e., using 2-phase multiferroic composites13,14,15,16,17,18,19,20,21,22,23,24,25,26,27,28. This can potentially be the basis of ultra-low-energy computing for our future information processing paradigm.
Results
Modeling
Switching dynamics of a single-domain poly-crystalline magnetostrictive particle in the presence of thermal fluctuations is modeled using the stochastic Landau-Lifshitz-Gilbert (LLG) equation29,30,31 that describes the time-evolution of the magnetization under various torques. There are three torques to consider here: torque due to shape anisotropy of the nanomagnet, torque due to generated stress anisotropy, and the torque associated with random thermal fluctuations. We consider a magnetostrictive single-domain32 nanomagnet made of polycrystalline Terfenol-D that is shaped like an elliptical cylinder. Fig. 2a shows the magnetization in three-dimensional space. We will call the z-axis the easy axis, the y-axis the in-plane hard axis, and the x-axis the out-of-plane hard axis based on the chosen dimensions of the nanomagnet. The two stable magnetization states are along the ± z-axis. In order to switch the magnetization, uniaxial compressive stress is applied in the z-direction.
In the macrospin approximation32,33,34,35,36,37, the magnetization M of the nanomagnet has a constant magnitude but a variable direction, so that we can represent it by a vector of unit norm where is the unit vector in the radial direction in spherical coordinate system represented by (r,θ,ϕ), θ [θ ∈ (0°, 180°)] is the polar angle, and ϕ [ϕ ∈ (0°, 360°)] is the azimuthal angle. Magnetization resides on the magnet's plane if ϕ = ±90° (y-z plane). The unit vectors associated with θ and ϕ rotations are and , respectively.
The total potential energy of the stressed nanomagnet is the sum of the shape anisotropy energy and stress anisotropy energy36 given by
where
Bshape(ϕ) is the ϕ-dependent strength of shape anisotropy energy (∝ cos2ϕ + constant term), which is minimum on the magnet's plane ϕ = ±90°, and Bstress is the strength of the stress anisotropy energy. (Details are provided in Supplementary Section S1.)
The torque due to shape and stress anisotropy is derived from the gradient of potential profile as
where Bshape,ϕ(ϕ) ∝ sin(2ϕ).
The torque due to thermal fluctuations is treated via a random magnetic field h expressed as
where hx, hy, and hz are the three components of h in x-, y-, and z-direction, respectively in Cartesian coordinates. We will assume the properties of the random field, h as described in Ref. 31.
The random thermal field can be expressed as31,37,38
where α is the phenomenological Gilbert damping parameter, γ is the gyromagnetic ratio of electrons, 1/Δt is proportional to the attempt frequency of the random thermal field, k is the Boltzmann constant, Δt is the simulation time-step, T is temperature, and G(0,1) is a Gaussian distribution with zero mean and unit standard deviation39. The simulation time-step Δt should be selected small enough so that decreasing that step further does not make any significant difference in the results. Accordingly, the thermal torque can be written as
where
Additionally, there is motion due to Gilbert damping29,30 (perpendicular to precessional motion) through which magnetization relaxes towards the minimum energy position in the magnet's potential landscape. The magnetization dynamics under the action of these two torques TE and TTH is described by the stochastic Landau-Lifshitz-Gilbert (LLG) equation as follows.
where α is the phenomenological Gilbert damping parameter and γ is the gyromagnetic ratio of electrons. Solving the above equation, we get the following coupled equations for the dynamics of θ and ϕ (see Supplementary Section S1 for detailed steps)
We will ignore the random thermal torque while explaining the basic magnetization dynamics, however, we will discuss the consequences of room-temperature thermal fluctuations with simulation results later. We will assume that the magnetization starts from (–z-axis) and the applied stress tries to switch it to (+z-axis).
Out-of-plane excursion of magnetization
First, we will intuitively describe how magnetization is deflected from its plane (ϕ = ±90°, i.e., y-z plane), and gets stabilized out-of-plane as depicted in Fig. 2b. Dependence of shape-anisotropy energy on azimuthal angle ϕ (rather than assuming ϕ = ±90°) generates additional motions of magnetization in and directions (see the motions containing the term Bshape,ϕ(ϕ) in Fig. 2c and equations (10) and (11)); both the components are proportional to sin(2ϕ) and vanish when ϕ = ±90°, but additionally the ϕ-component is proportional to the damping parameter α. As shown in the Fig. 2b, the applied stress produces a torque that tries to rotate the magnetization anticlockwise and forces it to reside out of magnet's plane. As magnetization is deflected from the plane of the magnet (ϕ = ±90°), the ϕ-component of the additional torque due to shape anisotropy as mentioned above [∝ α sin(2ϕ)] would try to bring the magnetization back to its plane. Because of such counteraction, out of the four quadrants for ϕ, the magnetization would be stable in the second or the fourth quadrant [i.e., (90°, 180°) or (270°, 360°)]. Note that sin(2ϕ) is negative in these two quadrants counteracting the precessional motion due to stress. We would call these two quadrants “good” quadrants and the other two (first and third) quadrants as “bad” quadrants, the reasoning behind which would be more transparent onwards. Consideration of the torques due to ϕ-dependence of shape anisotropy energy is central to the dynamics we present in this article. The important lesson to take away is that ϕ is stable only in “good” quadrants, which is why ϕ is much more likely to be in a “good” quadrant during switching.
Magnetization's motion in three-dimensional space
We will now describe the motion of magnetization intuitively under various torques originating from shape and stress anisotropy as shown in Fig. 2c. We intend the motion of magnetization to be along the direction since we are switching magnetization from towards . The precessional motion of magnetization due to torque generated by the applied stress is in the direction, but the damping of magnetization generates an additional motion, which is perpendicular to both the direction of magnetization () and , i.e., in direction. These two motions are depicted as and , respectively in Fig. 2c, where α is the damping parameter and the quantity B(ϕ) includes a term due to shape anisotropy Bshape(ϕ) in addition to the stress anisotropy term Bstress. The quantity Bstress is negative and it must beat the shape anisotropy term Bshape(ϕ) for switching to get started. Mathematically, note that both the quantities B(ϕ) and cosθ are negative in the interval 180° ≥ θ ≥ 90°. Hence, magnetization switches towards its desired direction due to the applied stress. However, this damped motion in direction is weak because of the multiplicative factor α, which is usually much less than one (e.g., α = 0.1 for Terfenol-D).
As magnetization rotates out-of-plane due to applied stress, and stays in a “good” quadrant for ϕ [i.e., (90°, 180°) or (270°, 360°)] as described earlier (Fig. 2b), it generates a motion of magnetization in the direction due to ϕ-dependence of shape anisotropy energy. Subsequently, a damped motion is generated too in the direction. These two motions are depicted as and , respectively in Fig. 2c, where Bshape,ϕ(ϕ) ∝ sin(2ϕ). Note that in the “good” quadrants for ϕ, Bshape,ϕ(ϕ) is negative. Thus, keeping the magnetization out of magnet's plane in a “good” quadrant is beneficial in switching the magnetization in its desired direction. In fact, it can eventually increase the switching speed by a couple of orders of magnitude. In case the magnetization resides out-of-plane but in a “bad” quadrant, it would have resisted the motion of magnetization in its desired direction of switching. A higher magnitude of stress keeps the magnetization out of magnet's plane, but more inside a “good” quadrant counteracting the random thermal kicks possibly acting in the opposite direction, however, the damped motion tries to bring the magnetization back towards the magnet's plane. As these two motions counteract each other (Fig. 2c), the magnetization keeps moving in the direction and eventually reaches the x-y plane (θ = 90°). Note that without damping, such counteraction does not happen and magnetization precesses alternatingly through “good” and “bad” quadrants.
Upon reaching at θ = 90°, if magnetization stays in a “good” quadrant for ϕ [i.e., (90°, 180°) or (270°, 360°)], the torque on the magnetization is in the correct direction so that it can traverse towards (Figs. 3a and 3b). This once again justifies of terminology (“good” or “bad”) used for the four quadrants of ϕ. Note that at θ = 90° (i.e., cos θ = 0), the effect of stress on the magnetization rotation has diminished completely. The only two motions that are active at that point are and (Fig. 2c). Since α ≪ 1, magnetization quickly gets out of the θ = 90° position and as the magnetization vector gets deflected from θ = 90° towards θ = 0°, the effect of stress comes into play.
Stress cycle, magnetization directions, and potential profiles
The stress-cycle alongwith the energy profiles and magnetization directions at different instants of time during switching of magnetization is shown in the Fig. 4. At time t0, the magnetization direction is along the easy axis and the potential landscape of the nanomagnet is unperturbed by stress. The potential profile of the magnet is ‘symmetric’ in both θ- and ϕ-space with two degenerate minima at θ = 0°, 180° and a maximum at θ = 90° in θ-space. The anisotropy in the barrier is due to shape anisotropy only, which is ~ 44 kT at room-temperature using the magnet's dimensions and material parameters for Terfenol-D (Supplementary Table S1, Refs. 40,41,42,43,44). Note that the barrier height separating the two stable states (θ = 0° and 180°) is meant when the magnetization resides in-plane (i.e., ϕ = ±90°) of the magnet. The barrier goes higher when the magnetization is deflected from ϕ = 90° as shown in Fig. 4c (at time t0). The barrier is highest when the magnetization points along the out-of-plane direction (ϕ = 0° or 180°), which is due to the small thickness of the nanomagnet compared to the lateral dimensions. Magnetization can start from any angle ϕinitial ∈ (0°, 360°) in the presence of thermal noise (Supplementary Fig. S2).
As a compressive stress is ramped up on the nanomagnet between time instants t0 and t1, the potential landscape in θ-space becomes monostable near ϕ = ±90° provided a sufficient stress is applied. The potential barrier near ϕ = 0° or 180° may not become monostable in θ-space since the barrier height is high therein, however, that is not necessary for switching. Since application of stress rotates the magnetization in ϕ-direction, it can eventually come near ϕ = ±90° and starts switching from towards θ = 90° (Supplementary Fig. S3). The minimum energy position between time instants t1 and t2 is at (θ = 90°, ϕ = ±90°). From Fig. 4c, we can see that the potential profile at time instant t1 is still ‘symmetric’.
Stress is held constant between time instants t1 and t2, and the magnetization eventually reaches the x-y plane (θ = 90°). For a fast enough ramp rate and high enough stress, magnetization will reside in a “good” quadrant as explained before. This will dictate that magnetization traverses in the correct direction towards θ = 0°. A fast enough ramp rate will facilitate that the magnetization does not backtrack even after crossing θ = 90° towards θ = 0°. If stress is held constant for a longer time, the magnetization would have higher tendency to collapse on the magnet's plane following which thermal fluctuations may scuttle the magnetization either in a “good” quadrant or in a “bad” quadrant, making the success rate 50%.
Note that we reverse the stress (compression to tensile) between time instants t2 and t4 rather than just withdrawing it, which makes the potential landscape of the nanomagnet more steep in θ-space. But, it does not necessarily mean that the switching will be completed always faster since reversal of stress can cause magnetization to traverse into “bad” quadrants in ϕ-space causing magnetization to precess and switching delay may be eventually increased. Such increase in switching delay may happen particularly for higher stress levels. However, reversing the stress makes the success rate of switching a bit (<5%) higher in the presence of thermal fluctuations. The tensile stress is held constant and when θ becomes ≤ 5°, switching is deemed to have completed. The stress is withdrawn at the end between time instants t5 and t6 to complete the switching process.
Magnetization dynamics
Fig. 5 plots the magnetization dynamics for different values of ϕinitial (while keeping fixed values of θinitial, stress, and ramp rate) to depict the significance of out-of-plane excursion of magnetization. For Figs. 5a and 5b, the magnetization initially lies in the plane of the magnet (ϕinitial = ±90°) and precessional motion of magnetization due to applied stress is in the direction, which increases ϕ with time. Thus, the magnetization starts out in the “good” quadrant. Note that both the motions of magnetization (damped motion due to applied stress and the motion due to out-of-plane excursion depicted as and , respectively in the Fig. 2c) are in the direction so θ decreases with time and the magnetization rotates in the correct direction towards θ = 90°. The increasing out-of-plane excursion of the magnetization vector due to ϕ increasing with time however is opposed by the damped motion due to out-of-plane excursion (depicted as in Fig. 2c), which tries to bring the magnetization back to the magnet's plane. These two effects quickly balance and ϕ assumes a stable value in the “good” quadrant as seen in the plots (the flat regions of the ϕ-plots). When θ reaches 90°, the torque due to stress and shape anisotropy vanishes. At this point, we start to reverse the stress and the damped motion due to stress and shape anisotropy eventually becomes again in the direction. That continues to rotate the magnetization in the right direction towards θ = 0°, ending in successful switching. Slightly past 0.4 ns, continuing ϕ-rotation because of precessional motion due to stress and shape anisotropy pushes ϕ into a “bad” quadrant, but eventually it escapes into the other “good” quadrant. This brief excursion into the “bad” quadrant causes the ripple in θ-plots.
For Figs. 5c and 5d, the magnetization vector is initially lifted far out of the magnet's plane (ϕinitial = 0°, 180°), where the huge out-of-plane shape anisotropy cannot be overcome by the stress anisotropy and B(ϕ) becomes positive, i.e., |Bstress| < |Bshape(ϕ)|. So magnetization precesses in the clockwise direction () rather than in the anticlockwise direction (). Thus ϕ decreases with time, which immediately takes magnetization inside a “good” quadrant and eventually |Bstress| becomes greater than |Bshape(ϕ)|. Then ϕ assumes a stable value because of the damped motion due to out-of-plane excursion (depicted as in Fig. 2c). Afterwards, switching occurs similarly for the cases as in Figs. 5a and 5b. Slightly past 0.3 ns, continuing ϕ rotation pushes ϕ into a “bad” quadrant, but eventually it escapes into the other good quadrant. Once again, this brief excursion into the bad quadrant causes the ripple in θ-plots and switching is completed successfully at the end.
Switching failures
Fig. 6 demonstrates a couple of examples when switching fails. In Fig. 6a, when the polar angle θ reaches 90°, the azimuthal angle ϕ has ventured into the “bad” quadrant (0°,90°). Thus, switching eventually fails. In Fig. 6b, when the polar angle θ reaches 90°, the azimuthal angle ϕ is greater than 90° and hence is in a “good” quadrant. However, after reaching , the magnetization backtracks to the initial state and switching fails. This happens because of the long ramp duration bringing ϕ into the “bad” quadrant (0°,90°) and also during the passage of long duration thermal fluctuations have ample opportunity to scuttle the switching. Such switching failure is depicted intuitively in the Fig. 7 and explained below.
As magnetization leaves from θ = 90° towards and stress is ramped down, the torque due to stress tries to rotate the azimuthal angle ϕ of magnetization clockwise rather than anticlockwise (mathematically note that cosθ is positive for 90° ≥ θ ≥ 0° and B(ϕ) is still negative when stress has not been brought down significantly, i.e., still |Bstress| > |Bshape(ϕ)|). For a slow ramp-rate this rotation may be considerable and magnetization can stray into a “bad” quadrant. Moreover, thermal fluctuations can aggravate the scenario. Switching may impede and magnetization vector can backtrack towards causing a switching failure. In this way, switching failure may happen even after the magnetization has crossed the hard axis (θ = 90°) towards its destination (Fig. 7), which is why it does require a fast enough ramp rate during the ramp-down phase of stress. This is an intriguing phenomenon, which comes out after analyzing the magnetization dynamics in a complete three dimensional potential landscape.
Successful switching rates with respect to stress and ramp rate
Fig. 8 plots the successful switching rates at room-temperature (300 K) when the magnetostrictive nanomagnet is subjected to stress between 10 MPa and 30 MPa with ramp duration (60 ps, 90 ps, and 120 ps) as a parameter. A moderately large number (10,000) of simulations were performed for each value of stress and ramp duration to generate these results. Initial angle distributions at 300 K for both θ and ϕ are taken into account during simulations (Supplementary Fig. S2). The minimum stress needed to switch the magnetization at 0 K is ~ 5 MPa, but the minimum stress needed to ensure switching at 300 K is ~ 14 MPa for 60 ps ramp duration and ~ 17 MPa for 90 ps ramp duration. The minimum stress of 5 MPa is attributed to the removal of in-plane shape anisotropy energy barrier by the stress anisotropy, while the increase of stress at 300 K is due to scuttling of magnetization in “bad” quadrants due to increased thermal fluctuations. When the ramp duration is longer, a higher stress is required to prevent magnetization traversing into “bad” quadrants. Hence, it is better to reduce the ramp duration (i.e., a faster ramp rate) to increase the success rate of switching at a lower stress level. Simulation results show that with 1 ps ramp duration, the critical stress reduces by ~ 2 MPa compared to the case of 60 ps ramp duration.
For 120 ps ramp duration, ~ 100% success probability is unattainable for any value of stress since thermal agitations have higher latitude to divert the magnetization in wrong direction while stress is ramped down; at higher stresses accompanied by a long ramp duration, there occurs higher out-of-plane excursion pushing the magnetization in “bad” quadrants, which further aggravates the error probability. At very long ramp duration, the success (and error) probability becomes 50%, since the magnetization would stay in-plane of the magnet and during the ramp-down phase, random thermal fluctuations may equally scuttle the magnetization either in the “good” quadrants or in the ‘bad” quadrants.
Supplementary Figs. S4 and S5 plot the different statistical distributions of switching delay for 15 MPa applied stress with 60 ps ramp duration. The mean and maximum switching delay as plotted in the distribution (Supplementary Fig. S5) are 0.52 ns and 1.13 ns, respectively.
Discussion
Therefore, we require the following two criteria for successful switching without creating any asymmetry in the potential landscape even in the presence of thermal fluctuations: (1) a high enough stress that keeps the magnetization more out-of-plane inside the good quadrants; and (2) a fast enough ramp rate that reduces the possibility of backtracking of magnetization while it is crossing (or even after crossing) the hard axis (θ = 90°) towards its destination. A high stress and a fast ramp rate also increase the switching speed and surpass the detrimental effects of thermal fluctuations.
In conclusion, we have shown that binary switching in a symmetric potential landscape is feasible, even in the presence of thermal noise. We have theoretically demonstrated such possibility in successful magnetization reversal of a single magnetostrictive particle, however, the ramification of our study is not limited to the field of nanomagnetism or to the particular shape or material used for the specimen. The out-of-plane dynamics plays the crucial role to ensure such error-resilient switching. This can open up a new methodology of binary switching since tilting the potential landscape would not be necessary and we hope that our findings would stimulate experimental research to establish the proposed methodology of binary switching.
Methods
We have solved the stochastic Landau-Lifshitz-Gilbert (LLG) equation29,30,31, which describes the time-evolution of magnetization vector in the presence of various torques including a torque due to random thermal fluctuations. Analytical expressions of different torques are mathematically formulated and incorporated in the stochastic LLG equation. Then the expressions of non-linear dynamics are derived analytically by solving the stochastic LLG equation in spherical coordinate system. Subsequently the expressions are numerically solved to get the simulation results. Detailed analytical steps are provided in the Supplementary Section S1.
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Acknowledgements
This work was supported by the U.S. National Science Foundation under Nanoelectronics for 2020 and Beyond (NEB) grant ECCS-1124714 and by the Semiconductor Research Corporation under the Nanoelectronics Research Initiative (NRI) Task 2203.001.
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K.R. conceived the idea, performed the simulations, and wrote the paper. S.B. and J.A. commented on the manuscript. All authors discussed the results and agreed to the conclusions of the paper.
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Roy, K., Bandyopadhyay, S. & Atulasimha, J. Binary switching in a ‘symmetric’ potential landscape. Sci Rep 3, 3038 (2013). https://doi.org/10.1038/srep03038
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DOI: https://doi.org/10.1038/srep03038
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npj Computational Materials (2017)
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Fast 180° magnetization switching in a strain-mediated multiferroic heterostructure driven by a voltage
Scientific Reports (2016)
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