Featured
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Article |
Inverse chirality-induced spin selectivity effect in chiral assemblies of π-conjugated polymers
The authors report the inverse effect of chiral-induced spin selectivity in an organic material.
- Rui Sun
- , Kyung Sun Park
- & Dali Sun
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Article
| Open AccessShallow defects and variable photoluminescence decay times up to 280 µs in triple-cation perovskites
Quantifying recombination in halide perovskites is crucial, but quantitative analysis remains rare. Here the authors observe a long-lived and continuously changing photoluminescence decay time due to the high density of shallow defects and substantial rates of charge carrier trapping.
- Ye Yuan
- , Genghua Yan
- & Thomas Kirchartz
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Research Briefing |
Vibrational optical control via cation motions in perovskite solar cells
Hybrid organic–inorganic perovskite materials have promise as the photovoltaic technology of the future. A method for spectroscopic optical control reveals how the structural dynamics and vibrations of a perovskite’s organic cations affect the electronic performance of working photovoltaic devices.
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Research Briefing |
Near-ideal in-memory sensing and computing devices using ferroelectrics
A compact, time- and energy-efficient computing architecture — based on ferroelectric-defined reconfigurable two-dimensional photodiode arrays — is shown to be capable of in-memory sensing and computing.
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Comment |
The organic electrochemical transistor conundrum when reporting a mixed ionic–electronic transport figure of merit
An essential part of developing organic mixed ionic–electronic conducting materials and organic electrochemical transistors is consistent and standardized reporting of the product of charge carrier mobility and volumetric capacitance, the μC* product. This Comment argues that unexpected changes in transistor channel resistance can overestimate this figure of merit, leading to a confusion of comparisons in the literature.
- Maryam Shahi
- , Vianna N. Le
- & Alexandra F. Paterson
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News & Views |
Designer quantum dot molecules and beyond
Quantum dots couple to form artificial molecules that allow for variable colour emission in response to an electric field.
- James Cassidy
- , Justin Ondry
- & Dmitri V. Talapin
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Article |
Electric-field-induced colour switching in colloidal quantum dot molecules at room temperature
Current quantum dot emitters are limited to small-spectral-range colour tuning accompanied by intensity reduction. Electric-field-induced reversible emission colour switching without intensity loss can be achieved on a single-particle level in quantum dot molecules with two coupled emission centres.
- Yonatan Ossia
- , Adar Levi
- & Uri Banin
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Article |
Single-molecule photoelectron tunnelling spectroscopy
The transmission spectrum reflects energy alignment between electrodes and frontier orbitals in single-molecule junctions but few experimental tools exist for characterization beyond the HOMO–LUMO gap. Here, the authors develop a single-molecule photoelectron tunnelling spectroscopy approach that makes it possible to map the transmission spectrum beyond the HOMO–LUMO gap at room temperature.
- Haojie Liu
- , Lijue Chen
- & Wenjing Hong
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Letter |
Giant magnon spin conductivity in ultrathin yttrium iron garnet films
The authors report the observation of an enhanced magnon conductivity close to the two-dimensional transport regime in ultrathin yttrium iron garnet.
- X.-Y. Wei
- , O. Alves Santos
- & B. J. van Wees
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Article |
Tapered fibertrodes for optoelectrical neural interfacing in small brain volumes with reduced artefacts
Here the authors fabricate a fibre-coupled electrode ‘fibertrode’ that integrates light emission sites and platinum microelectrodes on tapered optical fibre neural implants, for combined stimulation and recording of neural activity over small brain volumes in vivo with reduced photoelectric artefacts.
- Barbara Spagnolo
- , Antonio Balena
- & Ferruccio Pisanello
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Article |
Single-junction organic solar cells with over 19% efficiency enabled by a refined double-fibril network morphology
The morphology of donor–acceptor blends in organic photovoltaics dictates the efficiency of the exciton dissociation and charge diffusion, and thus the final device performance. Here, the authors show that filament assembly helps to maximize the output, further enabling a power conversion efficiency greater than 19%.
- Lei Zhu
- , Ming Zhang
- & Feng Liu
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News & Views |
Precision doping to heal traps
Passivation of traps via site-specific surface doping allows access to the intrinsic properties of organic semiconductors and leads to the observation of electron atmospheres in organic crystals.
- Oana D. Jurchescu
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Perspective |
Perovskite semiconductors for room-temperature exciton-polaritonics
An outlook on the potential of lead-halide perovskites as a playground for exciton-polariton studies and for the development of polaritonic devices operating at room temperature is provided.
- Rui Su
- , Antonio Fieramosca
- & Qihua Xiong
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News & Views |
Hot plasmons make graphene shine
Bright hot plasmon emission is observed in graphene due to the ultrafast relaxation of hot carriers that were excited by femtosecond laser pulses of visible light.
- Frank H. L. Koppens
- & Klaas-Jan Tielrooij
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Perspective |
Semimetals for high-performance photodetection
Semimetal photodetectors provide high-speed and broadband operation but suffer from serious drawbacks such as high dark currents. This Perspective discusses the opportunities offered by topological effects to overcome these issues and improve their performance.
- Jing Liu
- , Fengnian Xia
- & Dong Sun
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Letter |
Magnetic proximity and nonreciprocal current switching in a monolayer WTe2 helical edge
The coupling between magnetism and topology is studied in a van der Waals heterostructure.
- Wenjin Zhao
- , Zaiyao Fei
- & David H. Cobden
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Letter |
Black phosphorus as a bipolar pseudospin semiconductor
Anisotropic honeycomb crystal of black phosphorous is found to have pseudospin polarization greater than 95% at room temperature, attributed to the merging of Dirac cones. This bipolar pseudospin semiconductor may be useful for pseudospintronics.
- Sung Won Jung
- , Sae Hee Ryu
- & Keun Su Kim
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Article |
Tunable room-temperature spin galvanic and spin Hall effects in van der Waals heterostructures
Enhanced spin-charge conversion in graphene is realized by proximity coupling to WS2 and electric-field tunability is demonstrated.
- L. Antonio Benítez
- , Williams Savero Torres
- & Sergio O. Valenzuela
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Letter |
Electrical switching in a magnetically intercalated transition metal dichalcogenide
A remarkably low critical current is found to reorient the magnetic order in a magnetically intercalated transition metal dichalcogenide, suggesting this class of materials could form a basis for antiferromagnetic spintronics.
- Nityan L. Nair
- , Eran Maniv
- & James G. Analytis
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Letter |
A window to trap-free charge transport in organic semiconducting thin films
Water clusters induce hole traps in organic semiconductor thin films. Detrimental effects of hole and electron traps on charge transport can be avoided by using materials with ionization energy and electron affinity within an energy window of 2.4 eV.
- Naresh B. Kotadiya
- , Anirban Mondal
- & Gert-Jan A. H. Wetzelaer
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Letter |
Granular aluminium as a superconducting material for high-impedance quantum circuits
A fluxonium qubit is constructed out of granular aluminium, revealing its potential for superconducting quantum technologies.
- Lukas Grünhaupt
- , Martin Spiecker
- & Ioan M. Pop
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Letter |
Emissive and charge-generating donor–acceptor interfaces for organic optoelectronics with low voltage losses
Charge-transfer states with comparable recombination and charge-splitting rates are shown to be a key ingredient for donor–acceptor organic blends that perform well in both light-emitting and photovoltaic applications.
- Sascha Ullbrich
- , Johannes Benduhn
- & Koen Vandewal
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Letter |
Emergence of quantum correlations from interacting fibre-cavity polaritons
Two-photon correlation measurements in a resonantly excited fibre-cavity polariton system stay below the classical limit for zero time delay, suggesting quantum correlations between the polaritons.
- Guillermo Muñoz-Matutano
- , Andrew Wood
- & Thomas Volz
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Perspective |
Electrolyte-based ionic control of functional oxides
Electrolyte gating of complex oxides enables substantial control of electronic phase transitions, allowing electrical control of complex phenomena. Here, the role of both electrostatic and electrochemical mechanisms in this process is elucidated.
- Chris Leighton
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Article |
Electric-field induced structural transition in vertical MoTe2- and Mo1–xWxTe2-based resistive memories
A vertical electric field is shown to induce reversible transitions between a semiconducting 2H phase, a distorted transient structure and a conducting Td phase in MoTe2 and Mo1–xWxTe2 multilayers, and used to realize vertical resistive random access memories.
- Feng Zhang
- , Huairuo Zhang
- & Joerg Appenzeller
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Article |
Design rules for minimizing voltage losses in high-efficiency organic solar cells
Key optoelectronic properties for donor and acceptor organic semiconductors are identified to obtain organic solar cells with reduced open-circuit voltage losses and high power conversion efficiencies.
- Deping Qian
- , Zilong Zheng
- & Feng Gao
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Article |
Electron–phonon interaction in efficient perovskite blue emitters
Films of exfoliated crystals of two-dimensional hybrid metal halide perovskites with phenyl groups as organic cations show increased molecular rigidity, reduced electron–phonon interactions and blue emission with photoluminescence quantum yield approaching 80%.
- Xiwen Gong
- , Oleksandr Voznyy
- & Edward H. Sargent
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News & Views |
At the flick of a switch
Voltage control of recently discovered two-dimensional magnets has been demonstrated, highlighting their potential for low-power data storage.
- Ajit Srivastava
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Article |
Universal strategy for Ohmic hole injection into organic semiconductors with high ionization energies
It is shown that Ohmic contacts for the injection of hole carriers into organic semiconductors with high ionization energy can be formed by adding ultrathin interlayers with higher ionization energy.
- Naresh B. Kotadiya
- , Hao Lu
- & Gert-Jan A. H. Wetzelaer
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Commentary |
Critical assessment of charge mobility extraction in FETs
Mobility is an important charge-transport parameter in organic, inorganic and hybrid semiconductors. We outline some of the common pitfalls of mobility extraction from field-effect transistor (FET) measurements and propose practical recommendations to avoid reporting erroneous mobilities in publications.
- Hyun Ho Choi
- , Kilwon Cho
- & Vitaly Podzorov
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Review Article |
Energy conversion approaches and materials for high-efficiency photovoltaics
This Review describes the sunlight conversion strategies — and their technological implementations — that are currently being investigated to realize solar cells with efficiencies beyond the Shockley–Queisser limit.
- Martin A. Green
- & Stephen P. Bremner
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Article |
Reducing the efficiency–stability–cost gap of organic photovoltaics with highly efficient and stable small molecule acceptor ternary solar cells
Ternary organic blends using two non-fullerene acceptors are shown to improve the efficiency and stability of low-cost solar cells based on P3HT and of high-performance photovoltaic devices based on low-bandgap donor polymers.
- Derya Baran
- , Raja Shahid Ashraf
- & Iain McCulloch
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Article |
Tailoring exchange couplings in magnetic topological-insulator/antiferromagnet heterostructures
Heterostructures formed by the magnetic topological insulator Cr-doped (Bi,Sb)2Te and the antiferromagnet CrSb are shown to exhibit emergent interfacial magnetic phenomena that can be tuned with the heterostructure geometry.
- Qing Lin He
- , Xufeng Kou
- & Kang L. Wang
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Letter |
Thermoelectric detection and imaging of propagating graphene plasmons
A device is presented that can detect mid-infrared plasmons in graphene encapsulated by hexagonal boron nitride via the thermoelectric effect; the natural decay product of the plasmons (electronic heat) is converted into a measurable voltage signal.
- Mark B. Lundeberg
- , Yuanda Gao
- & Frank H. L. Koppens
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News & Views |
Electrical spin switching
Ultra-low-power electronic switching of stable exciton–polariton spin states has now been achieved in a semiconductor microcavity. This opens a new route to the integration of spin-based photonics and electronics.
- T. C. H. Liew
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Article |
Exploring the origin of high optical absorption in conjugated polymers
The photocurrent generated in organic photodetectors and solar cells can be enhanced by increasing light absorption in the active layer. It is now shown that an extended persistence length can increase the oscillator strength of conjugated polymers.
- Michelle S. Vezie
- , Sheridan Few
- & Jenny Nelson
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News & Views |
Skyrmionics gets hot
The observation of magnetic skyrmions at room temperature that can be driven by short current pulses at speeds exceeding 100 m s−1 raises great expectations for skyrmion-based racetrack memories.
- Stefan Krause
- & Roland Wiesendanger
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Article |
Elimination of charge carrier trapping in diluted semiconductors
By diluting conjugated polymers in high-bandgap host matrices it is shown that electron trapping effects can be significantly reduced. This approach is used to fabricate polymer LEDs with enhanced efficiency and reduced fabrication costs.
- D. Abbaszadeh
- , A. Kunz
- & P. W. M. Blom
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Article |
Robust reconfigurable electromagnetic pathways within a photonic topological insulator
Topologically protected states at the interface of magnetic domain walls in a parallel plate waveguide with adjustable rods, are shown to be directed along different paths, as the waveguide geometry changes.
- Xiaojun Cheng
- , Camille Jouvaud
- & Alexander B. Khanikaev
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Article |
Conductance saturation in a series of highly transmitting molecular junctions
The conductance of single-molecule junctions based on oligoacenes is shown to saturate when the molecule length increases. The saturation trend depends on the frontier orbitals of the metals used and on their hybridization with molecular π-orbitals.
- T. Yelin
- , R. Korytár
- & O. Tal
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Article |
Correlated metals as transparent conductors
Electronic many-body effects are used to control the electron effective mass, and thus the plasma energy and electrical conductivity, of thin films of the correlated metals SrVO3 and CaVO3, making them good candidates as transparent conductors.
- Lei Zhang
- , Yuanjun Zhou
- & Roman Engel-Herbert
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Letter |
Time-domain separation of optical properties from structural transitions in resonantly bonded materials
Femtosecond optical spectroscopy and single-shot electron diffraction measurements during the photoinduced amorphization of the phase-change material Ge2Sb2Te5 demonstrate that optical properties can be separated from the structural state.
- Lutz Waldecker
- , Timothy A. Miller
- & Simon Wall
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News & Views |
Solving a wonderful problem
Superconducting qubits are used to demonstrate features of quantum fault tolerance, making an important step towards the realization of a practical quantum machine.
- Simon Benjamin
- & Julian Kelly
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Letter |
Universal helimagnon and skyrmion excitations in metallic, semiconducting and insulating chiral magnets
The resonant microwave excitation response of metals, semiconductors and insulating chiral magnets is studied by examining their entire magnetic phase diagrams, which includes the skyrmion lattice phase. A unified model to explain this response is also developed.
- T. Schwarze
- , J. Waizner
- & D. Grundler
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Article |
Room-temperature antiferromagnetic memory resistor
Magnetic memory devices are typically based on ferromagnetic materials. Now, a memory resistor based on the antiferromagnetic alloy FeRh is demonstrated at room temperature.
- X. Marti
- , I. Fina
- & R. Ramesh
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News & Views |
Quantum engineering
A series of breakthroughs is making the fabrication of single-atom devices possible. Their behaviour is controlled by the quantum state of single dopants, and they hold promise for applications such as quantum bits, magnetometers and memories.
- Joaquin Fernández Rossier