News & Views |
Featured
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News & Views |
Slow on, fast off
The slow turn-on speed in accumulation-mode organic electrochemical transistors is explained by asymmetric ion transport in switching kinetics.
- Hang Yu
- & Jenny Nelson
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Article
| Open AccessElectrochemically actuated microelectrodes for minimally invasive peripheral nerve interfaces
Electrode arrays for neurological diagnosis and treatment carry a risk of nerve injury. Nerve cuffs with tiny voltage-controlled shape-reconfigurable electrode arrays have been reported, allowing active wrapping around delicate nerves.
- Chaoqun Dong
- , Alejandro Carnicer-Lombarte
- & George G. Malliaras
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Article |
Understanding asymmetric switching times in accumulation mode organic electrochemical transistors
The turn-off time is generally faster than the turn-on time in accumulation mode organic electrochemical transistors (OECTs), but the mechanism is less understood. Here the authors find different transient behaviours of turn-on and turn-off in accumulation mode OECTs, and ion transport is the limiting factor of device kinetics.
- Jiajie Guo
- , Shinya E. Chen
- & David S. Ginger
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Perspective |
Potential and challenges of computing with molecular materials
Molecular materials for computing progress intensively but the performance and reliability still lag behind. Here the authors assess the current state of computing with molecular-based materials and describe two issues as the basis of a new computing technology: continued exploration of molecular electronic properties and process development for on-chip integration.
- R. Stanley Williams
- , Sreebrata Goswami
- & Sreetosh Goswami
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News & Views |
Chromogenic identification of breakdown
Early detection of electrical degradation can be identified by colour change due to the chromogenic response of blended molecules in dielectric polymers.
- Gregory A. Sotzing
- & Pritish S. Aklujkar
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Article |
Monolithic 3D integration of 2D materials-based electronics towards ultimate edge computing solutions
Monolithic 3D integration of electronics based on fully 2D materials is demonstrated in the performance of artificial intelligence tasks.
- Ji-Hoon Kang
- , Heechang Shin
- & Sang-Hoon Bae
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Article |
Autonomous indication of electrical degradation in polymers
Early detection of electrical degradation in dielectric polymers is crucial but remains challenging. A general strategy of blending the polymer with chromogenic molecules is reported, which generates a visually discernible colour change as chemically activated by oxygen radicals generated in situ, indicating the early stage of electrical degradation in polymers.
- Xiaoyan Huang
- , Shuai Zhang
- & Jinliang He
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Research Briefing |
Physical reservoir computers that can adapt to perform different tasks
A traditional physical-reservoir device has limited flexibility and cannot perform well across a range of computing tasks, owing to the fixed reservoir properties of the physical system. However, by exploiting the rich magnetic phase spaces of a single chiral magnet, reservoir properties can be reconfigured. This control enables on-demand optimization of computational performance across diverse machine-learning tasks.
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Article |
Scalable integration of hybrid high-κ dielectric materials on two-dimensional semiconductors
A van der Waals buffer layer of Sb2O3 enables the integration of high-κ dielectric layer with sub-1 nm equivalent oxide thickness on two-dimensional semiconductors, resulting in high performance of two-dimensional field-effect transistors.
- Yongshan Xu
- , Teng Liu
- & Tianyou Zhai
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Article |
3D printable high-performance conducting polymer hydrogel for all-hydrogel bioelectronic interfaces
A bi-continuous hydrogel prepared from phase-separated PEDOT:PSS and polyurethane is 3D printed into soft biolelectronic devices with high electrical conductivity, stretchability and toughness for long-term in vivo electrophysiological monitoring and stimulation.
- Tao Zhou
- , Hyunwoo Yuk
- & Xuanhe Zhao
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Article |
Observation of anti-damping spin–orbit torques generated by in-plane and out-of-plane spin polarizations in MnPd3
The authors address spin–orbit torques and magnetization switching in MnPd3/CoFeB hetrostructures.
- Mahendra DC
- , Ding-Fu Shao
- & Shan X. Wang
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News & Views |
Artificial neuron transmits chemical signals
An artificial neuron architecture based on antiambipolar organic electrochemical transistors shows responses to biological ions and neurotransmitters akin to real neurons with comparable speed. The soft and more biocompatible nature of organic semiconductors could enable applications in brain–machine interfaces and in vivo sensing.
- Shinya E. Chen
- , Rajiv Giridharagopal
- & David S. Ginger
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Review Article |
Coherent antiferromagnetic spintronics
This Review discusses the field of antiferromagnetic spintronics with a focus on coherent effects.
- Jiahao Han
- , Ran Cheng
- & Shunsuke Fukami
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Article
| Open AccessIon-tunable antiambipolarity in mixed ion–electron conducting polymers enables biorealistic organic electrochemical neurons
Silicon-based complementary metal-oxide semiconductors or negative differential resistance device circuits can emulate neural features, yet are complicated to fabricate and not biocompatible. Here, the authors report an ion-modulated antiambipolarity in mixed ion–electron conducting polymers demonstrating capability of sensing, spiking, emulating the most critical biological neural features, and stimulating biological nerves in vivo.
- Padinhare Cholakkal Harikesh
- , Chi-Yuan Yang
- & Simone Fabiano
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Article |
High-entropy enhanced capacitive energy storage
Electrostatic capacitors can enable ultrafast energy storage and release, but advances in energy density and efficiency need to be made. Here, by doping equimolar Zr, Hf and Sn into Bi4Ti3O12 thin films, a high-entropy stabilized Bi2Ti2O7 pyrochlore phase forms with an energy density of 182 J cm−3 and 78% efficiency.
- Bingbing Yang
- , Yang Zhang
- & Yuan-Hua Lin
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Article |
Tapered fibertrodes for optoelectrical neural interfacing in small brain volumes with reduced artefacts
Here the authors fabricate a fibre-coupled electrode ‘fibertrode’ that integrates light emission sites and platinum microelectrodes on tapered optical fibre neural implants, for combined stimulation and recording of neural activity over small brain volumes in vivo with reduced photoelectric artefacts.
- Barbara Spagnolo
- , Antonio Balena
- & Ferruccio Pisanello
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Article |
Gate-tuneable and chirality-dependent charge-to-spin conversion in tellurium nanowires
All-electrical generation, manipulation and detection of spin polarization in chiral nanowires is demonstrated.
- Francesco Calavalle
- , Manuel Suárez-Rodríguez
- & Luis E. Hueso
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Article |
Memristive control of mutual spin Hall nano-oscillator synchronization for neuromorphic computing
This allows versatile non-volatile tuning of the mutual synchronization of chains of up to four oscillators and provides a path toward individual oscillator control in large oscillatory arrays.
- Mohammad Zahedinejad
- , Himanshu Fulara
- & Johan Åkerman
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News & Views |
The secret order of disorder
A seemingly disordered network of nanowires governed by thermodynamics is used as the physical ‘reservoir’ in a memristive implementation of reservoir computing to process spatiotemporal information.
- Qiangfei Xia
- , J. Joshua Yang
- & Rivu Midya
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Why it Matters |
Quantum engineers in high demand
Gabriele Rainò, Lukas Novotny and Martin Frimmer discuss the approach they are pursuing at ETH Zürich to provide students with an education in quantum engineering.
- Gabriele Rainò
- , Lukas Novotny
- & Martin Frimmer
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Article |
Band gap engineering in blended organic semiconductor films based on dielectric interactions
Changes in dielectric constant due to intimate mixing of thiophene molecules with different gaps between ionization energy and electron affinity induce gap variations at the single-particle level, finely tunable by controlling the mixture ratio.
- Katrin Ortstein
- , Sebastian Hutsch
- & Karl Leo
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Article |
Efficient and low-voltage vertical organic permeable base light-emitting transistors
Vertical organic light-emitting transistors are realized by using a porous base electrode in the centre of the device, which improves efficiency and reduces operating voltage by regulating charge transport and forming an optical microcavity.
- Zhongbin Wu
- , Yuan Liu
- & Karl Leo
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Article |
Permeable superelastic liquid-metal fibre mat enables biocompatible and monolithic stretchable electronics
Coating of liquid metals on electrospun elastomeric fibre mats leads to the realization of conducting buckled meshes that can be stretched up to 1,800% strain while preserving both stable electrical properties and permeability to air and moisture.
- Zhijun Ma
- , Qiyao Huang
- & Zijian Zheng
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Article |
Creation of moiré bands in a monolayer semiconductor by spatially periodic dielectric screening
The moiré pattern that is formed between well-aligned graphene and hexagonal boron nitride can modify the properties of WSe2 (placed close by without intentional angle alignment), leading to the formation of a mini Brillouin zone and the folding of the bands in WSe2.
- Yang Xu
- , Connor Horn
- & Kin Fai Mak
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News & Views |
Optical switches and modulators in deep freeze
The integration of silicon-based waveguides with barium titanate thin films enables the realization of efficient electro-optic switches and modulators operating at cryogenic temperatures, offering promising opportunities for quantum technologies.
- Goran Z. Mashanovich
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News & Views |
Lighting up soft robotics
A transparent, high-permittivity elastomeric dielectric material shows potential for light-emitting soft robots and stretchable optoelectronics that can self-heal.
- Jonathan Rossiter
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Article |
A transparent, self-healing and high-κ dielectric for low-field-emission stretchable optoelectronics
Stretchable and self-healing light-emitting capacitors operating at low frequency and low voltage have been realized using a transparent elastomeric dielectric with high permittivity.
- Yu Jun Tan
- , Hareesh Godaba
- & Benjamin C. K. Tee
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Article |
Titanium-carbide MXenes for work function and interface engineering in perovskite solar cells
Addition of MXenes in the halide perovskite film, in the electron transport layer and at the interface between these layers is shown to enhance the efficiency of and reduce hysteresis in perovskite solar cells.
- A. Agresti
- , A. Pazniak
- & A. Di Carlo
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Article |
Nanometre-thin indium tin oxide for advanced high-performance electronics
Controlled physical vapour deposition of indium tin oxide layers with thickness down to 4 nm allows the use of these materials as active channels in high-performing transistors for digital and radiofrequency electronics.
- Shengman Li
- , Mengchuan Tian
- & Yanqing Wu
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Comment |
Integrating graphene into semiconductor fabrication lines
Electronic and photonic devices based on graphene have unique properties, leading to outstanding performance figures of merit. Mastering the integration of this unconventional material into an established semiconductor fabrication line represents a critical step towards commercialization.
- Daniel Neumaier
- , Stephan Pindl
- & Max C. Lemme
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Review Article |
Memristive crossbar arrays for brain-inspired computing
Memristive devices show great potential as artificial synapses and neurons, yet brain-inspired computing can be realized only by integrating a large number of these devices into reliable arrays. This Review discusses the challenges in the integration and use in computation of large-scale memristive neural networks.
- Qiangfei Xia
- & J. Joshua Yang
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Article |
Hybrid photoelectrochemical and photovoltaic cells for simultaneous production of chemical fuels and electrical power
Solar energy is widely used for fuel production and energy storage, but the majority of photoelectrochemical cells cannot operate without an external power source. A device for simultaneous and direct production of renewable fuels and electrical power is now proposed.
- Gideon Segev
- , Jeffrey W. Beeman
- & Ian D. Sharp
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News & Views |
Electrically detecting infrared light
Researchers have developed a graphene plasmonics detector that is suitable for fast-response and high-resolution detection of infrared photons at room temperature.
- Zhe Fei
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Article |
Efficient electrical detection of mid-infrared graphene plasmons at room temperature
A system of patterned graphene nanoresonators/nanoribbons can be used as an efficient mid-infrared detector, based on plasmonic resonant absorption and subsequent carrier thermalization.
- Qiushi Guo
- , Renwen Yu
- & Fengnian Xia
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Article |
Insight into doping efficiency of organic semiconductors from the analysis of the density of states in n-doped C60 and ZnPc
The doping efficiency of n-type molecular dopants in organic semiconductors is shown to depend on the energy difference between the electron affinity of the host and the ionization potential of the doped system.
- Christopher Gaul
- , Sebastian Hutsch
- & Frank Ortmann
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Article |
Beating the thermodynamic limit with photo-activation of n-doping in organic semiconductors
The activation of cleavable organometallic dimers upon exposure to ultraviolet radiation allows air-stable n-type doping of organic materials with electron affinity lower than the expected thermodynamic reducing strength of the dimers.
- Xin Lin
- , Berthold Wegner
- & Antoine Kahn
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Article |
Solution-based electrical doping of semiconducting polymer films over a limited depth
A solution process for the diffusion of dopants in organic semiconducting films over a limited depth has been developed. The method is applied to single polymers and donor–acceptor mixtures, and for the realization of single-layer solar cells.
- Vladimir A. Kolesov
- , Canek Fuentes-Hernandez
- & Bernard Kippelen
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News & Views |
Prime time
In the past decade, artificial materials with unusual wave interactions have significantly evolved and matured. In honour of the tenth anniversary of the premiere metamaterials conference, we look at the directions in which this field is evolving, and its impact on technology.
- Andrea Alù
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Article |
Localized dielectric breakdown and antireflection coating in metal–oxide–semiconductor photoelectrodes
Silicon-based photoelectrodes are attractive for solar fuel production, but suffer from vulnerability to corrosion. Using dielectric breakdown, a generic approach to improve the performance of metal-oxide semiconductor photoelectrodes is proposed.
- Li Ji
- , Hsien-Yi Hsu
- & Edward T. Yu
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Commentary |
Robots with a sense of touch
Tactile sensors provide robots with the ability to interact with humans and the environment with great accuracy, yet technical challenges remain for electronic-skin systems to reach human-level performance.
- Chiara Bartolozzi
- , Lorenzo Natale
- & Giorgio Metta
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Review Article |
Metal oxides for optoelectronic applications
Optical transparency, tunable conducting properties and easy processability make metal oxides key materials for advanced optoelectronic devices. This Review discusses recent advances in the synthesis of these materials and their use in applications.
- Xinge Yu
- , Tobin J. Marks
- & Antonio Facchetti
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Article |
Correlated metals as transparent conductors
Electronic many-body effects are used to control the electron effective mass, and thus the plasma energy and electrical conductivity, of thin films of the correlated metals SrVO3 and CaVO3, making them good candidates as transparent conductors.
- Lei Zhang
- , Yuanjun Zhou
- & Roman Engel-Herbert
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Article |
Flexible high power-per-weight perovskite solar cells with chromium oxide–metal contacts for improved stability in air
The use of a chromium oxide interlayer separating the perovskite film from the metal contacts improves the stability of perovskite solar cells in air. Deposited on thin plastic foils, these ultralight devices power model airplanes and dirigibles.
- Martin Kaltenbrunner
- , Getachew Adam
- & Siegfried Bauer
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Letter |
Hybrid optical–electrical detection of donor electron spins with bound excitons in silicon
A scheme of hybrid optical–electrical detection of an ensemble of donor electrons bound to phosphorus in silicon reveals electron spin Rabi oscillations and long coherence times, setting the foundations for a single-electron spin read-out technique.
- C. C. Lo
- , M. Urdampilleta
- & J. J. L. Morton
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Article |
Synthesis of ultrathin polymer insulating layers by initiated chemical vapour deposition for low-power soft electronics
Initiated chemical vapour deposition enables the conformal growth of ultrathin insulating polymer layers. These polymer films can be deposited on a broad range of materials used for organic and flexible electronics, including graphene.
- Hanul Moon
- , Hyejeong Seong
- & Sung Gap Im
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Article |
Atomic origin of ultrafast resistance switching in nanoscale electrometallization cells
Nanoscale resistance-switching cells that operate by means of electrochemical modification of metallic filaments are promising devices for post-CMOS electronics. Simulations of operating conductive cells are now used to describe electrochemical reactions.
- Nicolas Onofrio
- , David Guzman
- & Alejandro Strachan
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News & Views |
Cool electronics
Although heat removal in electronics at room temperature is typically governed by a hierarchy of conduction and convection phenomena, heat dissipation in cryogenic electronics can face a fundamental limit analogous to that of black-body emission of electromagnetic radiation.
- Jungwan Cho
- & Kenneth E. Goodson
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News & Views |
Negative capacitance detected
The experimental detection of negative capacitance in ferroelectrics rekindles hopes that the phenomenon could be used to further push the miniaturization of conventional transistors.
- Gustau Catalan
- , David Jiménez
- & Alexei Gruverman
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Letter |
Negative capacitance in a ferroelectric capacitor
Direct measurement of negative capacitance is now reported in a ferroelectric capacitor based on a thin, epitaxial ferroelectric PZT film.
- Asif Islam Khan
- , Korok Chatterjee
- & Sayeef Salahuddin