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Li-dendrite growth is an inherent problem for the application of Li-metal anodes in batteries. Here the authors coat the separator with functionalized nanocarbon with immobilized Li ions, regulating the dendrite growth direction and thereby improving the battery performance.
Electrochemical reduction of CO2 to CO is a route to synthesize fuels, but cheaper and more selective catalysts are required. Using a cell equipped with a bipolar membrane and the same Earth-abundant electrocatalyst at each electrode, Schreier et al. selectively produce CO, powered by a triple-junction photovoltaic.
Mixed matrix membranes can separate CO2 from flue gas mixtures but increasing selectivity without sacrificing permeability remains challenging. Selectivity can be increased with little loss in permeability by using nanoparticulate, amine-functionalized metal–organic framework fillers.
Electric vehicles are only as green as the electricity used to charge them, but owners tend to charge vehicles at times of peak use. This study shows that tailored emails increase engagement with information about time-of-use tariffs, with maximal effects within the first three months of ownership.
The presence of polysulfides in Li–S batteries is highly relevant to the battery performance, but their formation and evolution during battery operation are not well understood. Here the authors design an operando X-ray diffraction experiment to reveal their reaction mechanisms.
Development of electrocatalysts with high stability and activity is a critical challenge. Here, the authors combine simulations with in situ experiments to identify principles underlying simultaneously enhanced stability and activity of ultrathin (hydroxy)oxide films on transition metal substrates.
Organic compounds can be used as electrode materials for Li-ion batteries, but problems such as facile dissolution and low electrical conductivity hinder their application. Here the authors report π-conjugated quinoxaline-based heteroaromatic molecules with multiple redox sites to tackle the problems.
The most efficient silicon solar cells use interdigitated back-contact silicon heterojunction architectures. Here, the authors fabricate this type of cell via a simpler process, using an interband silicon tunnel junction for the electron contact and reaching a certified efficiency higher than 22%.
Shale gas and oil production and prospective development are increasing, but methods for shale extraction (‘fracking’) have been met with opposition. This study shows that informed discourse around shale development focussed on risks or doubts about benefits in a similar manner across the US and UK.
The conversion efficiency of organic solar cells suffers from their low open-circuit voltages. Here, the authors expose a link between electron-vibrations coupling and non-radiative recombinations, derive a new limit for the efficiency of organic solar cells, and redefine their optimal optical gap.
High shares of variable energy sources will require different operational modes for dispatchable generation. Schill et al. explore the impact of increased wind and solar power on the German electricity system and find that the number of start-ups grows by 81% while its cost increases by 119% by 2030.
Multiple exciton generation has been shown to improve the performance of quantum-dot-based solar cells. Yan et al. now apply it to photoinduced hydrogen production and present a system using PbS quantum-dot photoelectrodes that yields an external quantum efficiency of over 100%.
Fast ionic conductivity of solid electrolytes is a must in the development of next-generation solid-electrolyte-based lithium-ion batteries. Here the authors report that composite polymer electrolytes with well-aligned inorganic nanowires can achieve much larger conductivities than those without.
Nuclear accidents generate vast echoes in public opinion, and often determine policy decisions to suspend nuclear programs. This study shows the unintended implications of nuclear plant shutdown in Tennessee Valley between 1983 and 1986, demonstrating deleterious consequences for public health.
Thin-film photovoltaic devices are often based on toxic or rare materials. Here, Wang et al. grow oriented Sb2Se3 thin film on a ZnO buffer layer, and fabricate solar cells with a certified 5.9% conversion efficiency and which pass harsh stability tests under humidity, heat and illumination.
To tackle the high energy consumption of buildings, information programs to promote investment in energy efficiency measures have been introduced. This study compares the effectiveness of three US programs and finds that despite large energy savings, progress is lacking for small and medium sized buildings.
Photoelectrochemical devices based on III–V semiconductors have high performance potential but their cost and stability inhibit their wide application. Kang et al. make printed assemblies of GaAs-based photoelectrodes with separate optical and reactive interfaces, demonstrating water-splitting efficiency up to 13.1%.
Nanostructured black silicon can be used as a photoelectrode for solar-driven water splitting, but its high surface area can increase charge recombination and accelerate corrosion. Here the authors show that a thin, conformal film of TiO2 can increase both the photocurrent and the stability of black silicon.
The application of Li–O2 batteries is hindered by severe parasitic reactions in battery cycling. Here the authors show that the highly reactive singlet oxygen is the main cause for the electrolyte and carbon electrode degradation on discharge and charge.
Perovskite-based solar cells are often fabricated by methods that are not industrially scalable. Here, Yang et al. develop an ink formulation which gives similar devices by spin coating, the lab-scale standard, and blade coating, which is a more scalable, industry-relevant deposition method.